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Catherine Hirel - One of the best experts on this subject based on the ideXlab platform.

Jacques Pécaut - One of the best experts on this subject based on the ideXlab platform.

Dominique Luneau - One of the best experts on this subject based on the ideXlab platform.

Vefa Ahsen - One of the best experts on this subject based on the ideXlab platform.

Christine Anne Louise Watson - One of the best experts on this subject based on the ideXlab platform.

  • Development of a Scaleable Synthesis of a Geminal Dimethyl Tertiary Amine as an Inhaled Muscarinic Antagonist for the Treatment of COPD
    Organic Process Research & Development, 2012
    Co-Authors: Barry Richard Dillon, Dannielle F. Roberts, David A. Entwistle, Glossop Paul Alan, Craig J. Knight, Daniel Laity, Kim James, Céline F. B. Praquin, Strang Ross Sinclair, Christine Anne Louise Watson
    Abstract:

    An efficient and scalable process for the synthesis of muscarinic antagonist, PF-3635659 1, is described, illustrating redesign of an analogue-targeted synthesis which contained a scale-limiting rhodium-activated C–H amination step. The final route includes a reproducible modified Bouveault Reaction which has not previously been reported on a substrate of this complexity, or on such a scale with over 5 kg of the requisite gem-dimethylamine prepared via this methodology.

  • Development of a Scaleable Synthesis of a Geminal Dimethyl Tertiary Amine as an Inhaled Muscarinic Antagonist for the Treatment of COPD
    2012
    Co-Authors: Barry Richard Dillon, Dannielle F. Roberts, David A. Entwistle, Daniel Laity, Kim James, Céline F. B. Praquin, Paul A. Glossop, Craig J. Knight, Ross S. Strang, Christine Anne Louise Watson
    Abstract:

    An efficient and scalable process for the synthesis of muscarinic antagonist, PF-3635659 1, is described, illustrating redesign of an analogue-targeted synthesis which contained a scale-limiting rhodium-activated C–H amination step. The final route includes a reproducible modified Bouveault Reaction which has not previously been reported on a substrate of this complexity, or on such a scale with over 5 kg of the requisite gem-dimethylamine prepared via this methodology