The Experts below are selected from a list of 303 Experts worldwide ranked by ideXlab platform
Hua Zuo - One of the best experts on this subject based on the ideXlab platform.
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Smiles rearrangement for the synthesis of diarylamines
Arkivoc, 2011Co-Authors: Xiao Tian, Gang Liu, He-lin Wei, Hao Yang, Li-ying Wang, Hua ZuoAbstract:A protocol for the one-pot synthesis of diarylamines via Smiles rearrangement under microwave irradiation has been developed. Various diarylamines were effectively synthesized starting from readily available substituted phenols, arylamines and Chloroacetyl Chloride in moderate to good yields (58–92%).
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A Facile C-N BondFormation: One-Pot Reaction of Phenols and Amines via Smiles Rearrangement
Synlett, 2010Co-Authors: Hao Yang, Xiao Tian, Li-ying Wang, Dong-soo Shin, Jia-zhou Zhou, Hong-bo Qiao, Hua ZuoAbstract:Diarylamines and arylalkylamines were synthesized in high yields from 2-chlorophenols and amines, activated by Chloroacetyl Chloride under microwave irradiation (20―60 min) or conventional thermal conditions (3―6 h). The key transformation is believed to proceed via Smiles rearrangement by initial O-alkylation and subsequent cyclization.
P.k. Dubey - One of the best experts on this subject based on the ideXlab platform.
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A validated CE method for determining dimethylsulfate a carcinogen and Chloroacetyl Chloride a potential genotoxin at trace levels in drug substances.
Journal of pharmaceutical and biomedical analysis, 2011Co-Authors: Muzaffar Khan, K. Jayasree, K.v.s.r. Krishna Reddy, P.k. DubeyAbstract:A simple and rapid capillary zone electrophoretic method was developed for determining dimethyl sulfate a possible human carcinogen and mutagen and Chloroacetyl Chloride a potential genotoxic agent at trace levels in pharmaceutical drug substances by indirect photometric detection. A systematic screening of various anionic probes was performed to obtain the best separation conditions and sensitivity. High sensitivities with low quantification and detection levels were achieved for dimethylsulfate and Chloroacetyl Chloride using a background electrolyte (BGE) containing 5 mM pyridine dicarboxylic acid as the probe ion. The method is specific, precise and accurate for the two genotoxins. The optimized method was validated for specificity, precision, linearity, accuracy and stability in solution. Calibration curves were linear (R>0.999) for both dimethylsulfate and Chloroacetyl Chloride in the range LOQ - 300% of nominal concentrations. The CE method was effectively implemented for estimating dimethylsulfate and Chloroacetyl Chloride in two different active pharmaceutical ingredients (APIs).
Hao Yang - One of the best experts on this subject based on the ideXlab platform.
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Smiles rearrangement for the synthesis of diarylamines
Arkivoc, 2011Co-Authors: Xiao Tian, Gang Liu, He-lin Wei, Hao Yang, Li-ying Wang, Hua ZuoAbstract:A protocol for the one-pot synthesis of diarylamines via Smiles rearrangement under microwave irradiation has been developed. Various diarylamines were effectively synthesized starting from readily available substituted phenols, arylamines and Chloroacetyl Chloride in moderate to good yields (58–92%).
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A Facile C-N BondFormation: One-Pot Reaction of Phenols and Amines via Smiles Rearrangement
Synlett, 2010Co-Authors: Hao Yang, Xiao Tian, Li-ying Wang, Dong-soo Shin, Jia-zhou Zhou, Hong-bo Qiao, Hua ZuoAbstract:Diarylamines and arylalkylamines were synthesized in high yields from 2-chlorophenols and amines, activated by Chloroacetyl Chloride under microwave irradiation (20―60 min) or conventional thermal conditions (3―6 h). The key transformation is believed to proceed via Smiles rearrangement by initial O-alkylation and subsequent cyclization.
Jerry Tso - One of the best experts on this subject based on the ideXlab platform.
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Trace level determination of Chloroacetyl Chloride and degradation products by derivatization gas chromatography.
Journal of pharmaceutical and biomedical analysis, 2017Co-Authors: Marie-france Morissette, Larry Wigman, Jerry TsoAbstract:A gas chromatographic procedure has been developed for the trace determination of Chloroacetyl Chloride (CAC) and two of its impurities: methyl chloroacetate (MCA) and chloroacetic acid (CAA). All three compounds are derivatized using piperidine in dichloroethane prior to their analysis via gas chromatography coupled with a flame ionization detection (GC-FID). Recoveries of each compound were assessed in two different pharmaceutical matrices (intermediate and final active pharmaceutical ingredient) and ranged from 75 to 125%. The limit of quantitation has been determined to be 0.10% wt/wt for CAA and 0.03% wt/wt for CAC and MCA. The linearity ranged from 0.03 to 5.00% wt/wt for CAC and MCA and from 0.10 to 5.00% wt/wt for CAA, with correlation coefficients from 0.9995 to 1.0000. Repeatability was evaluated at LOQ and at 5.00% wt/wt and was found to be between 1.4-3.0%.
Pragati Sharma - One of the best experts on this subject based on the ideXlab platform.
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Solvent‐free cycloaddition reaction of 3‐indolylimines with Chloroacetyl Chloride under microwave irradiation
Heteroatom Chemistry, 2003Co-Authors: Anshu Dandia, Ruby Singh, Pragati SharmaAbstract:Solvent-free approach is developed for the rapid synthesis of spiro[azetidine-indoles] 6a–g on basic alumina supported potassium carbonate (K2CO3–Al2O3) from the cycloaddition reaction of indolylimines 3 and Chloroacetyl Chloride 4 as synthons using microwaves. The procedure neither required toxic and hazardous base nor volatile solvents. 3 was synthesized in situ by the neat reaction of indole-2,3-diones 1 and fluorinated anilines 2 under microwave irradiation. Solvent-free aminoalkylation of spiro compounds 6a and 6b has been carried out under microwaves. © 2003 Wiley Periodicals, Inc. Heteroatom Chem 14:468–473, 2003; Published online in Wiley InterScience (www.interscience.wiley.com). DOI 10.1002/hc.10180
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solvent free cycloaddition reaction of 3 indolylimines with Chloroacetyl Chloride under microwave irradiation
Heteroatom Chemistry, 2003Co-Authors: Anshu Dandia, Ruby Singh, Pragati SharmaAbstract:Solvent-free approach is developed for the rapid synthesis of spiro[azetidine-indoles] 6a–g on basic alumina supported potassium carbonate (K2CO3–Al2O3) from the cycloaddition reaction of indolylimines 3 and Chloroacetyl Chloride 4 as synthons using microwaves. The procedure neither required toxic and hazardous base nor volatile solvents. 3 was synthesized in situ by the neat reaction of indole-2,3-diones 1 and fluorinated anilines 2 under microwave irradiation. Solvent-free aminoalkylation of spiro compounds 6a and 6b has been carried out under microwaves. © 2003 Wiley Periodicals, Inc. Heteroatom Chem 14:468–473, 2003; Published online in Wiley InterScience (www.interscience.wiley.com). DOI 10.1002/hc.10180