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Anil K. Singh - One of the best experts on this subject based on the ideXlab platform.

  • Fluorescence Emission enhancement in substituted 3-styrylindoles in the solid state
    Journal of Luminescence, 2010
    Co-Authors: Abera Asefa, Anil K. Singh
    Abstract:

    Fluorescence Emission properties of substituted 3-styrylindoles viz 3-(2-phenylethenyl-E)-NH-indole (1), 3-[2-(4-cyanophenyl)ethenyl-E]-NH-indole (2), and 3-(2-cyano-2-phenylethenyl-Z]-NH-indole (3) in n-hexane, THF-H 2 O binary mixtures and solid state are reported. In general, Fluorescence efficiency in solid state is found to be much higher than in n-hexane solution. The Fluorescence enhancement in solid state is attributed to restricted intramolecular motions. Interestingly, the molecules of 3 in solid state are also bound together through intermolecular hydrogen bonds yielding polymer like structure, leading to further enhancement of Fluorescence Emission. In THF-H 2 O binary mixtures, drastic enhancement of Fluorescence efficiency is observed due to aggregate formation.

Mingxing Jin - One of the best experts on this subject based on the ideXlab platform.

Sethuraman Sankararaman - One of the best experts on this subject based on the ideXlab platform.

  • donor acceptor substituted phenylethynyltriphenylenes excited state intramolecular charge transfer solvatochromic absorption and Fluorescence Emission
    Beilstein Journal of Organic Chemistry, 2010
    Co-Authors: Ritesh Nandy, Sethuraman Sankararaman
    Abstract:

    Several 2-(phenylethynyl)triphenylene derivatives bearing electron donor and acceptor substituents on the phenyl rings have been synthesized. The absorption and Fluorescence Emission properties of these molecules have been studied in solvents of different polarity. For a given derivative, solvent polarity had minimal effect on the absorption maxima. However, for a given solvent the absorption maxima red shifted with increasing conjugation of the substituent. The Fluorescence Emission of these derivatives was very sensitive to solvent polarity. In the presence of strongly electron withdrawing (–CN) and strongly electron donating (–NMe2) substituents large Stokes shifts (up to 130 nm, 7828 cm−1) were observed in DMSO. In the presence of carbonyl substituents (–COMe and –COPh), the largest Stokes shift (140 nm, 8163 cm−1) was observed in ethanol. Linear correlation was observed for the Stokes shifts in a Lippert–Mataga plot. Linear correlation of Stokes shift was also observed with ET(30) scale for protic and aprotic solvents but with different slopes. These results indicate that the Fluorescence Emission arises from excited state intramolecular charge transfer in these molecules where the triphenylene chromophore acts either as a donor or as an acceptor depending upon the nature of the substituent on the phenyl ring. HOMO–LUMO energy gaps have been estimated from the electrochemical and spectral data for these derivatives. The HOMO and LUMO surfaces were obtained from DFT calculations.

  • Synthesis, Absorption, and FluorescenceEmission Properties of 1,3,6,8‐Tetraethynylpyrene and Its Derivatives
    European Journal of Organic Chemistry, 2005
    Co-Authors: Gandikota Venkataramana, Sethuraman Sankararaman
    Abstract:

    The synthesis of several 1,3,6,8-tetraethynylpyrene derivatives is reported. The effect of extended acetylenic conjugation on their absorption and Fluorescence-Emission properties is studied. Significant bathochromic shifts of both the absorption and Fluorescence Emission bands are observed. These derivatives emit Fluorescence in the visible (400–550 nm) region. (© Wiley-VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2005)

Abera Asefa - One of the best experts on this subject based on the ideXlab platform.

  • Fluorescence Emission enhancement in substituted 3-styrylindoles in the solid state
    Journal of Luminescence, 2010
    Co-Authors: Abera Asefa, Anil K. Singh
    Abstract:

    Fluorescence Emission properties of substituted 3-styrylindoles viz 3-(2-phenylethenyl-E)-NH-indole (1), 3-[2-(4-cyanophenyl)ethenyl-E]-NH-indole (2), and 3-(2-cyano-2-phenylethenyl-Z]-NH-indole (3) in n-hexane, THF-H 2 O binary mixtures and solid state are reported. In general, Fluorescence efficiency in solid state is found to be much higher than in n-hexane solution. The Fluorescence enhancement in solid state is attributed to restricted intramolecular motions. Interestingly, the molecules of 3 in solid state are also bound together through intermolecular hydrogen bonds yielding polymer like structure, leading to further enhancement of Fluorescence Emission. In THF-H 2 O binary mixtures, drastic enhancement of Fluorescence efficiency is observed due to aggregate formation.

Yuanfei Jiang - One of the best experts on this subject based on the ideXlab platform.