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Jaya Shree Anireddy - One of the best experts on this subject based on the ideXlab platform.

Edward R Biehl - One of the best experts on this subject based on the ideXlab platform.

  • facile synthesis of 2 substituted 4h 1 3 thiazines and 3 substituted 1 2 isothiazoles via benzyne intermediates
    Heterocycles, 2005
    Co-Authors: Hongming Zhang, Ramadas Sathunuru, Charles W Rees, Edward R Biehl
    Abstract:

    Substituted 2-dialkylamino-4H-1,3-benzothiazineswere Synthesizedby the reaction of (phenyl)[o-(trimethylsilyl)aryl]iodonium triflates and dialkyl-aminothiazadienes in the presence of 1.5 equivalent of Bu 4 NF. However, when these reactions were carried out in the presence of 4 equivalents of Bu 4 NF, 3-substituted 1,2-benzisothiazoles were obtained. Additionally, the reaction of phenyl[(3-trimethylsilyl)-2-naphthyl]iodonium triflate with dialkylaminothia-zadienes in the presence of Bu 4 NF gave 3-substituted 1,2-naphthisothiazoles. A possible mechaism for the latter reaction involving the trapping of a benzyne intermediate with a Nitrile Sulfide generated in situ by the reaction of dialkylaminothiazadiene, fluoride ion and trimethylsilyl fluoride is proposed.

Anjaiah Aitha - One of the best experts on this subject based on the ideXlab platform.

Manoranjan Behera - One of the best experts on this subject based on the ideXlab platform.

Satyanarayana Yennam - One of the best experts on this subject based on the ideXlab platform.