The Experts below are selected from a list of 179958 Experts worldwide ranked by ideXlab platform

Takehito Tsukinoki - One of the best experts on this subject based on the ideXlab platform.

Masashi Tashiro - One of the best experts on this subject based on the ideXlab platform.

Janet L Scott - One of the best experts on this subject based on the ideXlab platform.

  • understanding solid solid Organic Reactions
    Journal of the American Chemical Society, 2001
    Co-Authors: Gadi Rothenberg, Andrew P Downie, Colin L Raston, Janet L Scott
    Abstract:

    The concept of an Organic Reaction between two macroscopic solid particles is investigated. Thus, we study several Reactions that have been recently reported to proceed “in the solid phase” and clearly show that, in most cases, grinding the two solid reactants together results in the formation of a liquid phase. This is true both for catalytic transformations (e.g., aldol condensations and oligomerization of benzylic compounds) and for noncatalytic Reactions (Baeyer−Villiger oxidations, oxidative coupling of naphthols using iron chloride, condensation of amines and aldehydes to form azomethines, homo-etherification of benzylic alcohols using p-toluenesulfonic acid, and nuclear aromatic bromination with NBS). This liquefaction implies the existence of a eutectic mixture with Tfusion below ambient temperature (although both reagents have higher than ambient melting points). In cases where heating is required, it is again clear that a phase change (from solid to liquid) occurs, explaining the observed reacti...

Xinhe Bao - One of the best experts on this subject based on the ideXlab platform.

  • Applications of In Situ NMR in Catalytic Processes of Organic Reactions
    Current Organic Chemistry, 2001
    Co-Authors: Xiuwen Han, Zhimin Yan, Weiping Zhang, Xinhe Bao
    Abstract:

    In situ MAS NMR has been demonstrated to be a superior technique for analyzing desorbed reactants, reacting adsorbates, intermediates and products. The results are useful for getting deeper insights into catalytic processes and Reaction kinetics, and for revealing the mechanisms of Organic Reactions. The utility of in situ NMR spectroscopy has demonstrated that this technique is an important means for the studies of catalytic Organic Reactions. The objective of this paper is to give a review on the generation of apparatus for in situ MAS NMR experiments, and to illustrate the applications of the in situ MAS NMR techniques in various important Organic Reactions catalyzed by solid catalysts. The typical Reactions studied by in situ MAS NMR techniques include conversion of methanol to hydrocarbons (MTG process), aromatization of methane, ethylbenzene Reaction over zeolite HMOR. observation of carbenium intermediates formation, and photocatalytic Organic Reaction.

Satoko Nagashima - One of the best experts on this subject based on the ideXlab platform.