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Chanjuan Xi - One of the best experts on this subject based on the ideXlab platform.

Fei Wang - One of the best experts on this subject based on the ideXlab platform.

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Uwe Schilde - One of the best experts on this subject based on the ideXlab platform.

Na You - One of the best experts on this subject based on the ideXlab platform.

  • phase equilibria study of the benzene cyclohexane n n dimethylformamide Potassium Thiocyanate quaternary systems
    Fluid Phase Equilibria, 2014
    Co-Authors: Sha Song, Chunguang Lin, Na You
    Abstract:

    Abstract This work demonstrates the ability of N,N-dimethylformamide + Potassium Thiocyanate(DMF + KSCN) to act as a novel complex solvent for the removal of benzene from its mixture with cyclohexane. The (liquid + liquid) equilibria (LLE) were measured for a quaternary system of (DMF + KSCN + benzene + cyclohexane) under atmospheric pressure and at temperature 298.15 K. The tie-line data for quaternary mixtures of (DMF + KSCN + benzene + cyclohexane) are also presented. The selectivity coefficients from these LLE data were calculated and found to be better than those previously reported in the literature for the (DMF + benzene + cyclohexane) systems. Excellent correlation of data by the nonrandom two-liquid (NRTL) model was seen for the quaternary system and the predicted results were found to be in fairly good agreement with experimental data.

  • selection of internal standard for quantitative analysis of extraction of benzene from cyclohexane with n n dimethylformamide Potassium Thiocyanate complex solvent
    Chromatographia, 2014
    Co-Authors: Sha Song, Chunguang Lin, Na You
    Abstract:

    The use of novel complex solvents in liquid–liquid extraction of aromatic hydrocarbons has become an important aim in the petrochemical industry. Phase equilibrium data are necessary for the design, evaluation, and optimization of extraction processes that are based on phase equilibria. To detect the separation effect of benzene/cyclohexane mixtures accurately and obtain the phase equilibrium data, a fast and efficient liquid–liquid extraction method combined with internal-standard gas chromatography was established for the quantitative analysis of the extraction of benzene from cyclohexane with the N,N-dimethylformamide/Potassium Thiocyanate (DMF/KSCN) novel complex solvent. The phase separation phenomenon occurred in a quaternary (benzene/cyclohexane/DMF/KSCN) system. KSCN as a cosolvent to improve the selectivity of DMF was innovatively applied and there was no prior report of any quantitative analysis of this system. After repeated experiments, n-butyl alcohol was found to be a suitable internal standard. The proposed method exhibits good linearity with a coefficient of correlation ranging from 0.9982 to 0.9994. The limits of detection varied from 0.16 to 0.58 mg L−1. The recovery was from 90.91 to 109.44 %. The method achieved excellent reproducibility with interassay relative standard deviations of 1.9–7.1 %. Furthermore the accuracy and precision of the proposed method with DMF/KSCN as the extractant were compared with the same method with only DMF as the extractant. The results indicated that adding KSCN had no significant impact on this quantitative method, although the KSCN could not be detected by gas chromatography (the mass fraction of KSCN was calculated via mass balance). Liquid–liquid equilibrium data obtained from this proposed method also revealed that the DMF/KSCN complex solvent had a higher selectivity for benzene than that of only DMF. This method is suitable for routine quantification of benzene, cyclohexane, DMF, and KSCN with high precision and accuracy.