The Experts below are selected from a list of 1074 Experts worldwide ranked by ideXlab platform
Takao Tsuji - One of the best experts on this subject based on the ideXlab platform.
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Simple Method for Shiga Toxin 2e Purification by Affinity Chromatography via Binding to the Divinyl Sulfone Group
2016Co-Authors: Hideyuki Arimitsu, Keiko Sasaki, Hiroe Kojima, Tadashi Yanaka, Takao TsujiAbstract:Here we describe a simple affinity purification method for Shiga toxin 2e (Stx2e), a major causative factor of edema disease in swine. Escherichia coli strain MV1184 transformed with the expression plasmid pBSK-Stx2e produced Stx2e when cultivated in CAYE broth containing lincomycin. Stx2e bound to commercial D-galactose gel, containing α-D-galactose immobilized on agarose resin via a Divinyl Sulfone linker, and was eluted with phosphate-buffered saline containing 4.5 M MgCl2. A small amount of Stx2e bound to another commercial α-galactose-immobilized agarose resin, but not to β-galactose-immobilized resin. In addition, Stx2e bound to thiophilic adsorbent resin containing β-mercaptoethanol immobilized on agarose resin via a Divinyl Sulfone, and was purified in the same manner as from D-galactose gel, but the Stx2e sample contained some contamination. These results indicate that Stx2e bound to D-galactose gel mainly through the Divinyl Sulfone group on the resin and to a lesser extent through α-D-galactose. With these methods, the yields of Stx2e and attenuated mutant Stx2e (mStx2e) from 1 L of culture were approximately 36 mg and 27.7 mg, respectively, and the binding capacity of the D-galactose gel and thiophilic adsorbent resin for Stx2e was at least 20 mg per 1 ml of resin. In addition, using chimeric toxins with prototype Stx2 which did not bind to thiophilic adsorbent resin and some types of mutant Stx2e and Stx2 which contained inserted mutations in the B subunits, we found that, at the least, asparagine (amino acid 17 of the B subunits) was associate
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Simple method for Shiga toxin 2e purification by affinity chromatography via binding to the Divinyl Sulfone group.
PloS one, 2013Co-Authors: Hideyuki Arimitsu, Keiko Sasaki, Hiroe Kojima, Tadashi Yanaka, Takao TsujiAbstract:Here we describe a simple affinity purification method for Shiga toxin 2e (Stx2e), a major causative factor of edema disease in swine. Escherichia coli strain MV1184 transformed with the expression plasmid pBSK-Stx2e produced Stx2e when cultivated in CAYE broth containing lincomycin. Stx2e bound to commercial D-galactose gel, containing α-D-galactose immobilized on agarose resin via a Divinyl Sulfone linker, and was eluted with phosphate-buffered saline containing 4.5 M MgCl2. A small amount of Stx2e bound to another commercial α-galactose-immobilized agarose resin, but not to β-galactose-immobilized resin. In addition, Stx2e bound to thiophilic adsorbent resin containing β-mercaptoethanol immobilized on agarose resin via a Divinyl Sulfone, and was purified in the same manner as from D-galactose gel, but the Stx2e sample contained some contamination. These results indicate that Stx2e bound to D-galactose gel mainly through the Divinyl Sulfone group on the resin and to a lesser extent through α-D-galactose. With these methods, the yields of Stx2e and attenuated mutant Stx2e (mStx2e) from 1 L of culture were approximately 36 mg and 27.7 mg, respectively, and the binding capacity of the D-galactose gel and thiophilic adsorbent resin for Stx2e was at least 20 mg per 1 ml of resin. In addition, using chimeric toxins with prototype Stx2 which did not bind to thiophilic adsorbent resin and some types of mutant Stx2e and Stx2 which contained inserted mutations in the B subunits, we found that, at the least, asparagine (amino acid 17 of the B subunits) was associated with Stx2e binding to the Divinyl Sulfone group. The mStx2e that was isolated exhibited vaccine effects in ICR mice, indicating that these methods are beneficial for large-scale preparation of Stx2e toxoid, which protects swine from edema disease.
Jianfeng Wu - One of the best experts on this subject based on the ideXlab platform.
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Synthesis, Characterization, and Identification of New in Vitro Covalent DNA Adducts of Divinyl Sulfone, an Oxidative Metabolite of Sulfur Mustard
Chemical Research in Toxicology, 2017Co-Authors: Shanshan Lv, Yajiao Zhang, Yumei Zhao, Jia Chen, Hua Xu, Bin Xu, Jianfeng WuAbstract:Divinyl Sulfone (DVS) is an important oxidative metabolic product of sulfur mustard (SM) in vitro and in vivo. Although DVS is not a classical blister agent, its high reactivity and toxicity induced by vinyl groups can also cause blisters like SM upon contact with the skin, eyes, and respiratory organs. The purpose of this paper was to identify whether DVS could covalently bind to DNA bases to form new DNA adducts in cells in vitro. A series of adducts were synthesized and characterized using purine, nucleoside, or DNA, separately, as starting materials. The covalent site, pattern, and relative reactivity of adduct formation were identified and discussed in detail. The results showed that five high abundance site-specific DNA adducts, including two monoadducts and three cross-linked adducts, were obtained when DNA was used as a substrate. When HaCaT cells were exposed to 30 μM of DVS, four new DNA adducts containing monoadducts and cross-linked adducts were found and identified in cells, including N3-A mo...
Christian Slugovc - One of the best experts on this subject based on the ideXlab platform.
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Solvent-free macrocyclisation by nucleophile-mediated oxa-Michael addition polymerisation of Divinyl Sulfone and alcohols
Polymer Chemistry, 2017Co-Authors: Simone Strasser, Christina Wappl, Christian SlugovcAbstract:The oxa-Michael addition reaction has been widely studied and employed in organic synthesis, but has not been developed as a tool for polymer synthesis. Herein, the 4-dimethylaminopyridine initiated polyaddition reaction of Divinyl Sulfone and several di- or multifunctional alcohols has been studied. This atom-economical polymerisation reaction proceeds quickly and quantitatively under solvent-free conditions producing predominantly macrocyclic products following a zwitter-ionic mechanism. Multifunctional alcohols yield duroplastic polymers. Considering the ready availability of alcohols, the oxa-Michael addition polymerisation is an interesting alternative to the well-established thiol-Michael addition polymerisation.
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nucleophile mediated oxa michael addition reactions of Divinyl Sulfone a thiol free option for step growth polymerisations
Catalysis Science & Technology, 2015Co-Authors: Simone Strasser, Christian SlugovcAbstract:Triphenylphosphine and 4-dimethylaminopyridine promote the oxa-Michael addition reaction of alcohols and Divinyl Sulfone. Under solvent-free conditions, the reaction is particularly fast and allows for the preparation of polymers.
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Nucleophile-mediated oxa-Michael addition reactions of Divinyl Sulfone – a thiol-free option for step-growth polymerisations
Catalysis Science & Technology, 2015Co-Authors: Simone Strasser, Christian SlugovcAbstract:Triphenylphosphine and 4-dimethylaminopyridine promote the oxa-Michael addition reaction of alcohols and Divinyl Sulfone. Under solvent-free conditions, the reaction is particularly fast and allows for the preparation of polymers.
Hideyuki Arimitsu - One of the best experts on this subject based on the ideXlab platform.
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Simple Method for Shiga Toxin 2e Purification by Affinity Chromatography via Binding to the Divinyl Sulfone Group
2016Co-Authors: Hideyuki Arimitsu, Keiko Sasaki, Hiroe Kojima, Tadashi Yanaka, Takao TsujiAbstract:Here we describe a simple affinity purification method for Shiga toxin 2e (Stx2e), a major causative factor of edema disease in swine. Escherichia coli strain MV1184 transformed with the expression plasmid pBSK-Stx2e produced Stx2e when cultivated in CAYE broth containing lincomycin. Stx2e bound to commercial D-galactose gel, containing α-D-galactose immobilized on agarose resin via a Divinyl Sulfone linker, and was eluted with phosphate-buffered saline containing 4.5 M MgCl2. A small amount of Stx2e bound to another commercial α-galactose-immobilized agarose resin, but not to β-galactose-immobilized resin. In addition, Stx2e bound to thiophilic adsorbent resin containing β-mercaptoethanol immobilized on agarose resin via a Divinyl Sulfone, and was purified in the same manner as from D-galactose gel, but the Stx2e sample contained some contamination. These results indicate that Stx2e bound to D-galactose gel mainly through the Divinyl Sulfone group on the resin and to a lesser extent through α-D-galactose. With these methods, the yields of Stx2e and attenuated mutant Stx2e (mStx2e) from 1 L of culture were approximately 36 mg and 27.7 mg, respectively, and the binding capacity of the D-galactose gel and thiophilic adsorbent resin for Stx2e was at least 20 mg per 1 ml of resin. In addition, using chimeric toxins with prototype Stx2 which did not bind to thiophilic adsorbent resin and some types of mutant Stx2e and Stx2 which contained inserted mutations in the B subunits, we found that, at the least, asparagine (amino acid 17 of the B subunits) was associate
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Simple method for Shiga toxin 2e purification by affinity chromatography via binding to the Divinyl Sulfone group.
PloS one, 2013Co-Authors: Hideyuki Arimitsu, Keiko Sasaki, Hiroe Kojima, Tadashi Yanaka, Takao TsujiAbstract:Here we describe a simple affinity purification method for Shiga toxin 2e (Stx2e), a major causative factor of edema disease in swine. Escherichia coli strain MV1184 transformed with the expression plasmid pBSK-Stx2e produced Stx2e when cultivated in CAYE broth containing lincomycin. Stx2e bound to commercial D-galactose gel, containing α-D-galactose immobilized on agarose resin via a Divinyl Sulfone linker, and was eluted with phosphate-buffered saline containing 4.5 M MgCl2. A small amount of Stx2e bound to another commercial α-galactose-immobilized agarose resin, but not to β-galactose-immobilized resin. In addition, Stx2e bound to thiophilic adsorbent resin containing β-mercaptoethanol immobilized on agarose resin via a Divinyl Sulfone, and was purified in the same manner as from D-galactose gel, but the Stx2e sample contained some contamination. These results indicate that Stx2e bound to D-galactose gel mainly through the Divinyl Sulfone group on the resin and to a lesser extent through α-D-galactose. With these methods, the yields of Stx2e and attenuated mutant Stx2e (mStx2e) from 1 L of culture were approximately 36 mg and 27.7 mg, respectively, and the binding capacity of the D-galactose gel and thiophilic adsorbent resin for Stx2e was at least 20 mg per 1 ml of resin. In addition, using chimeric toxins with prototype Stx2 which did not bind to thiophilic adsorbent resin and some types of mutant Stx2e and Stx2 which contained inserted mutations in the B subunits, we found that, at the least, asparagine (amino acid 17 of the B subunits) was associated with Stx2e binding to the Divinyl Sulfone group. The mStx2e that was isolated exhibited vaccine effects in ICR mice, indicating that these methods are beneficial for large-scale preparation of Stx2e toxoid, which protects swine from edema disease.
Tanmaya Pathak - One of the best experts on this subject based on the ideXlab platform.
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first synthesis and antiprotozoal activities of Divinyl Sulfone modified carbohydrates
ChemInform, 2010Co-Authors: Tarun Kumar Pal, Tuli Dey, Arindam Chakrabarty, Debanjana Dey, Sudip Kumar Ghosh, Tanmaya PathakAbstract:Carbohydrate epoxides (I) react with mercaptoethanol (II) in a regiospecific fashion to afford the sulfides (III) which upon oxidation, mesylation, and elimination are converted into vinyl Sulfones (V).
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First Synthesis and Antiprotozoal Activities of Divinyl Sulfone‐Modified Carbohydrates.
ChemInform, 2010Co-Authors: Tarun Kumar Pal, Tuli Dey, Arindam Chakrabarty, Debanjana Dey, Sudip Kumar Ghosh, Tanmaya PathakAbstract:Carbohydrate epoxides (I) react with mercaptoethanol (II) in a regiospecific fashion to afford the sulfides (III) which upon oxidation, mesylation, and elimination are converted into vinyl Sulfones (V).
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First synthesis and antiprotozoal activities of Divinyl Sulfone-modified carbohydrates
Bioorganic & medicinal chemistry letters, 2010Co-Authors: Tarun Kumar Pal, Tuli Dey, Arindam Chakrabarty, Debanjana Dey, Sudip Kumar Ghosh, Tanmaya PathakAbstract:Divinyl Sulfone-modified carbohydrates have been synthesized for the first time by reacting easily available carbohydrate epoxides with thioethanol in a regiospecific fashion. One of the modified Divinyl Sulfones initiated significant cell death in Entamoeba species and the influence of the anomeric configurations on the biological activities of these sugar-derived Divinyl Sulfones has been highlighted. The most active compound in this series was found to be devoid of any toxicity.