Gallium Phosphide

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  • nanoscopic charge fluctuations in a Gallium Phosphide waveguide measured by single molecules
    2021
    Co-Authors: A B Shkarin, Simon Honl, Paul Seidler, Dominik Rattenbacher, Jan Renger, Tobias Utikal, Stephan Gotzinger, Vahid Sandoghdar
    Abstract:

    We present efficient evanescent coupling of single organic molecules to a Gallium Phosphide (GaP) subwavelength waveguide (nanoguide) decorated with microelectrodes. By monitoring their Stark shifts, we reveal that the coupled molecules experience fluctuating electric fields. We analyze the spectral dynamics of different molecules over a large range of optical powers in the nanoguide to show that these fluctuations are light-induced and local. A simple model is developed to explain our observations based on the optical activation of charges at an estimated mean density of $2.5\ifmmode\times\else\texttimes\fi{}{10}^{22}\text{ }\text{ }{\mathrm{m}}^{\ensuremath{-}3}$ in the GaP nanostructure. Our work showcases the potential of organic molecules as nanoscopic sensors of the electric charge as well as the use of GaP nanostructures for integrated quantum photonics.

  • optomechanics with one dimensional Gallium Phosphide photonic crystal cavities
    2019
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Dalziel J Wilson, Lukas Czornomaz, Paul Seidler
    Abstract:

    Gallium Phosphide offers an attractive combination of a high refractive index (n>3 for vacuum wavelengths up to 4 μm) and a wide electronic bandgap (2.26 eV), enabling optical cavities with small mode volumes and low two-photon absorption at telecommunication wavelengths. Heating due to strongly confined light fields is therefore greatly reduced. Here, we investigate the benefits of these properties for cavity optomechanics. Utilizing a recently developed fabrication scheme based on direct wafer bonding, we realize integrated one-dimensional photonic crystal cavities made of Gallium Phosphide with optical quality factors as high as 1.1×105. We optimize their design to couple the optical eigenmode at ∼200  THz via radiation pressure to a co-localized mechanical mode with a frequency of 3 GHz, yielding sideband-resolved devices. The high vacuum optomechanical coupling rate (g0=2π×400  kHz) permits amplification of the mechanical mode into the so-called mechanical lasing regime with input power as low as ∼20  μW. The observation of mechanical lasing implies a multiphoton cooperativity of C>1, an important threshold for the realization of quantum state transfer protocols. Because of the reduced thermo-optic resonance shift, optomechanically induced transparency can be detected at room temperature even in non-sideband-resolved devices in addition to the normally observed optomechanically induced absorption. Considering that GaP is also piezoelectric, these results establish GaP as an attractive material for future electro–opto-mechanical systems.

  • optomechanics with one dimensional Gallium Phosphide photonic crystal cavities
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Dalziel J Wilson, Lukas Czornomaz, Paul Seidler
    Abstract:

    Gallium Phosphide offers an attractive combination of a high refractive index ($n>3$ for vacuum wavelengths up to 4 {\mu}m) and a wide electronic bandgap (2.26 eV), enabling optical cavities with small mode volumes and low two-photon absorption at telecommunication wavelengths. Heating due to strongly confined light fields is therefore greatly reduced. Here, we investigate the benefits of these properties for cavity optomechanics. Utilizing a recently developed fabrication scheme based on direct wafer bonding, we realize integrated one-dimensional photonic crystal cavities made of Gallium Phosphide with optical quality factors as high as $1.1\times10^5$. We optimize their design to couple the optical eigenmode at $\approx 200$ THz via radiation pressure to a co-localized mechanical mode with a frequency of 3 GHz, yielding sideband-resolved devices. The high vacuum optomechanical coupling rate ($g_0=2\pi\times 400$ kHz) permits amplification of the mechanical mode into the so-called mechanical lasing regime with input power as low as $\approx 20$ {\mu}W. The observation of mechanical lasing implies a multiphoton cooperativity of $C>1$, an important threshold for the realization of quantum state transfer protocols. Because of the reduced thermo-optic resonance shift, optomechanically induced transparency can be detected at room temperature in addition to the normally observed optomechanically induced absorption.

  • integrated Gallium Phosphide nonlinear photonics
    2018
    Co-Authors: Dalziel J Wilson, Katharina Schneider, Simon Hoenl, Miles Anderson, Tobias J Kippenberg, Paul Seidler
    Abstract:

    Gallium Phosphide (GaP) is an indirect bandgap semiconductor used widely in solid-state lighting. Despite numerous intriguing optical properties---including large $\chi^{(2)}$ and $\chi^{(3)}$ coefficients, a high refractive index ($>3$), and transparency from visible to long-infrared wavelengths ($0.55-11\,\mu$m)---its application as an integrated photonics material has been little studied. Here we introduce GaP-on-insulator as a platform for nonlinear photonics, exploiting a direct wafer bonding approach to realize integrated waveguides with 1.2 dB/cm loss in the telecommunications C-band (on par with Si-on-insulator). High quality $(Q> 10^5)$, grating-coupled ring resonators are fabricated and studied. Employing a modulation transfer approach, we obtain a direct experimental estimate of the nonlinear index of GaP at telecommunication wavelengths: $n_2=1.2(5)\times 10^{-17}\,\text{m}^2/\text{W}$. We also observe Kerr frequency comb generation in resonators with engineered dispersion. Parametric threshold powers as low as 3 mW are realized, followed by broadband ($>100$ nm) frequency combs with sub-THz spacing, frequency-doubled combs and, in a separate device, efficient Raman lasing. These results signal the emergence of GaP-on-insulator as a novel platform for integrated nonlinear photonics.

  • Gallium Phosphide on silicon dioxide photonic devices
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Pol Welter, Herwig Hahn, Lukas Czornomaz, Paul Seidler
    Abstract:

    The development of integrated photonic circuits utilizing Gallium Phosphide requires a robust, scalable process for fabrication of GaP-on-insulator devices. Here, we present the first GaP photonic devices on SiO2. The process exploits direct wafer bonding of a GaP/Al x Ga1- x P/GaP heterostructure onto a SiO2-on-Si wafer followed by the removal of the GaP substrate and the Al x Ga1- x P stop layer. Photonic devices such as grating couplers, waveguides, and ring resonators are patterned by inductively coupled-plasma reactive-ion etching in the top GaP device layer. The peak coupling efficiency of the fabricated grating couplers is as high as −4.8 dB. Optical quality factors of 20 000 as well as second- and third-harmonic generation are observed with the ring resonators. Because the large bandgap of GaP provides for low two-photon absorption at telecommunication wavelengths, the high-yield fabrication of GaP-on-insulator photonic devices enabled by this work is especially interesting for applications in nanophotonics, where high quality factors or low mode volumes can produce high electric field intensities. The large bandgap also enables integrated photonic devices operating at visible wavelengths.

Katharina Schneider - One of the best experts on this subject based on the ideXlab platform.

  • optomechanics with one dimensional Gallium Phosphide photonic crystal cavities
    2019
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Dalziel J Wilson, Lukas Czornomaz, Paul Seidler
    Abstract:

    Gallium Phosphide offers an attractive combination of a high refractive index (n>3 for vacuum wavelengths up to 4 μm) and a wide electronic bandgap (2.26 eV), enabling optical cavities with small mode volumes and low two-photon absorption at telecommunication wavelengths. Heating due to strongly confined light fields is therefore greatly reduced. Here, we investigate the benefits of these properties for cavity optomechanics. Utilizing a recently developed fabrication scheme based on direct wafer bonding, we realize integrated one-dimensional photonic crystal cavities made of Gallium Phosphide with optical quality factors as high as 1.1×105. We optimize their design to couple the optical eigenmode at ∼200  THz via radiation pressure to a co-localized mechanical mode with a frequency of 3 GHz, yielding sideband-resolved devices. The high vacuum optomechanical coupling rate (g0=2π×400  kHz) permits amplification of the mechanical mode into the so-called mechanical lasing regime with input power as low as ∼20  μW. The observation of mechanical lasing implies a multiphoton cooperativity of C>1, an important threshold for the realization of quantum state transfer protocols. Because of the reduced thermo-optic resonance shift, optomechanically induced transparency can be detected at room temperature even in non-sideband-resolved devices in addition to the normally observed optomechanically induced absorption. Considering that GaP is also piezoelectric, these results establish GaP as an attractive material for future electro–opto-mechanical systems.

  • optomechanics with one dimensional Gallium Phosphide photonic crystal cavities
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Dalziel J Wilson, Lukas Czornomaz, Paul Seidler
    Abstract:

    Gallium Phosphide offers an attractive combination of a high refractive index ($n>3$ for vacuum wavelengths up to 4 {\mu}m) and a wide electronic bandgap (2.26 eV), enabling optical cavities with small mode volumes and low two-photon absorption at telecommunication wavelengths. Heating due to strongly confined light fields is therefore greatly reduced. Here, we investigate the benefits of these properties for cavity optomechanics. Utilizing a recently developed fabrication scheme based on direct wafer bonding, we realize integrated one-dimensional photonic crystal cavities made of Gallium Phosphide with optical quality factors as high as $1.1\times10^5$. We optimize their design to couple the optical eigenmode at $\approx 200$ THz via radiation pressure to a co-localized mechanical mode with a frequency of 3 GHz, yielding sideband-resolved devices. The high vacuum optomechanical coupling rate ($g_0=2\pi\times 400$ kHz) permits amplification of the mechanical mode into the so-called mechanical lasing regime with input power as low as $\approx 20$ {\mu}W. The observation of mechanical lasing implies a multiphoton cooperativity of $C>1$, an important threshold for the realization of quantum state transfer protocols. Because of the reduced thermo-optic resonance shift, optomechanically induced transparency can be detected at room temperature in addition to the normally observed optomechanically induced absorption.

  • integrated Gallium Phosphide nonlinear photonics
    2018
    Co-Authors: Dalziel J Wilson, Katharina Schneider, Simon Hoenl, Miles Anderson, Tobias J Kippenberg, Paul Seidler
    Abstract:

    Gallium Phosphide (GaP) is an indirect bandgap semiconductor used widely in solid-state lighting. Despite numerous intriguing optical properties---including large $\chi^{(2)}$ and $\chi^{(3)}$ coefficients, a high refractive index ($>3$), and transparency from visible to long-infrared wavelengths ($0.55-11\,\mu$m)---its application as an integrated photonics material has been little studied. Here we introduce GaP-on-insulator as a platform for nonlinear photonics, exploiting a direct wafer bonding approach to realize integrated waveguides with 1.2 dB/cm loss in the telecommunications C-band (on par with Si-on-insulator). High quality $(Q> 10^5)$, grating-coupled ring resonators are fabricated and studied. Employing a modulation transfer approach, we obtain a direct experimental estimate of the nonlinear index of GaP at telecommunication wavelengths: $n_2=1.2(5)\times 10^{-17}\,\text{m}^2/\text{W}$. We also observe Kerr frequency comb generation in resonators with engineered dispersion. Parametric threshold powers as low as 3 mW are realized, followed by broadband ($>100$ nm) frequency combs with sub-THz spacing, frequency-doubled combs and, in a separate device, efficient Raman lasing. These results signal the emergence of GaP-on-insulator as a novel platform for integrated nonlinear photonics.

  • Gallium Phosphide on silicon dioxide photonic devices
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Pol Welter, Herwig Hahn, Lukas Czornomaz, Paul Seidler
    Abstract:

    The development of integrated photonic circuits utilizing Gallium Phosphide requires a robust, scalable process for fabrication of GaP-on-insulator devices. Here, we present the first GaP photonic devices on SiO2. The process exploits direct wafer bonding of a GaP/Al x Ga1- x P/GaP heterostructure onto a SiO2-on-Si wafer followed by the removal of the GaP substrate and the Al x Ga1- x P stop layer. Photonic devices such as grating couplers, waveguides, and ring resonators are patterned by inductively coupled-plasma reactive-ion etching in the top GaP device layer. The peak coupling efficiency of the fabricated grating couplers is as high as −4.8 dB. Optical quality factors of 20 000 as well as second- and third-harmonic generation are observed with the ring resonators. Because the large bandgap of GaP provides for low two-photon absorption at telecommunication wavelengths, the high-yield fabrication of GaP-on-insulator photonic devices enabled by this work is especially interesting for applications in nanophotonics, where high quality factors or low mode volumes can produce high electric field intensities. The large bandgap also enables integrated photonic devices operating at visible wavelengths.

  • Gallium Phosphide microresonator frequency combs conference presentation
    2018
    Co-Authors: Simon Honl, Katharina Schneider, Dalziel J Wilson, Miles Anderson, Tobias J Kippenberg, Paul Seidler
    Abstract:

    Gallium Phosphide (GaP) is an attractive material for non-linear optics because of its broad transparency window (λ_vac > 548 nm) and large Kerr coefficient (n_2 ~ 6 × 10^-18 m^2/W). Though well-established in the semiconductor industry as a substrate for visible LEDs, its use in integrated photonics remains limited due to fabrication challenges. Recently we have developed a method to integrate high quality, epitaxially-grown GaP onto silica (SiO2) based on direct wafer bonding to an oxidized silicon carrier wafer. Here we exploit this platform to realize unprecedentedly low loss (Q > 3 × 10^5) GaP-on-SiO2 waveguide resonators which have been dispersion-engineered to support Kerr frequency comb generation in the C-band. Single-mode, grating-coupled ring resonators with radii from 10 – 100 μm are investigated. The threshold for parametric conversion is observed at input powers as little as 10 mW, followed by 0.1 – 1 THz frequency comb generation over a range exceeding 400 nm, in addition to strong second- and third-harmonic generation. Building on this advance, we discuss the prospects for low-noise, sub-mW-threshold soliton frequency combs with center frequencies tunable from the mid-IR to the near-IR. Applications of such devices range from precision molecular spectroscopy to ultrafast pulse generation to massively parallel coherent optical communication.

Peter G Schunemann - One of the best experts on this subject based on the ideXlab platform.

Jelena Vuckovic - One of the best experts on this subject based on the ideXlab platform.

Yannick Baumgartner - One of the best experts on this subject based on the ideXlab platform.

  • optomechanics with one dimensional Gallium Phosphide photonic crystal cavities
    2019
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Dalziel J Wilson, Lukas Czornomaz, Paul Seidler
    Abstract:

    Gallium Phosphide offers an attractive combination of a high refractive index (n>3 for vacuum wavelengths up to 4 μm) and a wide electronic bandgap (2.26 eV), enabling optical cavities with small mode volumes and low two-photon absorption at telecommunication wavelengths. Heating due to strongly confined light fields is therefore greatly reduced. Here, we investigate the benefits of these properties for cavity optomechanics. Utilizing a recently developed fabrication scheme based on direct wafer bonding, we realize integrated one-dimensional photonic crystal cavities made of Gallium Phosphide with optical quality factors as high as 1.1×105. We optimize their design to couple the optical eigenmode at ∼200  THz via radiation pressure to a co-localized mechanical mode with a frequency of 3 GHz, yielding sideband-resolved devices. The high vacuum optomechanical coupling rate (g0=2π×400  kHz) permits amplification of the mechanical mode into the so-called mechanical lasing regime with input power as low as ∼20  μW. The observation of mechanical lasing implies a multiphoton cooperativity of C>1, an important threshold for the realization of quantum state transfer protocols. Because of the reduced thermo-optic resonance shift, optomechanically induced transparency can be detected at room temperature even in non-sideband-resolved devices in addition to the normally observed optomechanically induced absorption. Considering that GaP is also piezoelectric, these results establish GaP as an attractive material for future electro–opto-mechanical systems.

  • optomechanics with one dimensional Gallium Phosphide photonic crystal cavities
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Dalziel J Wilson, Lukas Czornomaz, Paul Seidler
    Abstract:

    Gallium Phosphide offers an attractive combination of a high refractive index ($n>3$ for vacuum wavelengths up to 4 {\mu}m) and a wide electronic bandgap (2.26 eV), enabling optical cavities with small mode volumes and low two-photon absorption at telecommunication wavelengths. Heating due to strongly confined light fields is therefore greatly reduced. Here, we investigate the benefits of these properties for cavity optomechanics. Utilizing a recently developed fabrication scheme based on direct wafer bonding, we realize integrated one-dimensional photonic crystal cavities made of Gallium Phosphide with optical quality factors as high as $1.1\times10^5$. We optimize their design to couple the optical eigenmode at $\approx 200$ THz via radiation pressure to a co-localized mechanical mode with a frequency of 3 GHz, yielding sideband-resolved devices. The high vacuum optomechanical coupling rate ($g_0=2\pi\times 400$ kHz) permits amplification of the mechanical mode into the so-called mechanical lasing regime with input power as low as $\approx 20$ {\mu}W. The observation of mechanical lasing implies a multiphoton cooperativity of $C>1$, an important threshold for the realization of quantum state transfer protocols. Because of the reduced thermo-optic resonance shift, optomechanically induced transparency can be detected at room temperature in addition to the normally observed optomechanically induced absorption.

  • Gallium Phosphide on silicon dioxide photonic devices
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Pol Welter, Herwig Hahn, Lukas Czornomaz, Paul Seidler
    Abstract:

    The development of integrated photonic circuits utilizing Gallium Phosphide requires a robust, scalable process for fabrication of GaP-on-insulator devices. Here, we present the first GaP photonic devices on SiO2. The process exploits direct wafer bonding of a GaP/Al x Ga1- x P/GaP heterostructure onto a SiO2-on-Si wafer followed by the removal of the GaP substrate and the Al x Ga1- x P stop layer. Photonic devices such as grating couplers, waveguides, and ring resonators are patterned by inductively coupled-plasma reactive-ion etching in the top GaP device layer. The peak coupling efficiency of the fabricated grating couplers is as high as −4.8 dB. Optical quality factors of 20 000 as well as second- and third-harmonic generation are observed with the ring resonators. Because the large bandgap of GaP provides for low two-photon absorption at telecommunication wavelengths, the high-yield fabrication of GaP-on-insulator photonic devices enabled by this work is especially interesting for applications in nanophotonics, where high quality factors or low mode volumes can produce high electric field intensities. The large bandgap also enables integrated photonic devices operating at visible wavelengths.

  • Gallium Phosphide on silicon dioxide photonic devices
    2018
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Pol Welter, Herwig Hahn, Lukas Czornomaz, Paul Seidler
    Abstract:

    The development of integrated photonic circuits utilizing Gallium Phosphide requires a robust, scalable process for fabrication of GaP-on-insulator devices. Here we present the first GaP photonic devices on SiO$_2$. The process exploits direct wafer bonding of a GaP/Al$_x$Ga$_{1-x}$P/GaP heterostructure onto a SiO$_2$-on-Si wafer followed by removal of the GaP substrate and the Al$_x$Ga$_{1-x}$P stop layer. Photonic devices such as grating couplers, waveguides, and ring resonators are patterned by inductively coupled-plasma reactive-ion etching in the top GaP device layer. The peak coupling efficiency of the fabricated grating couplers is as high as 4.8 dB. Optical quality factors of 17000 as well as second- and third-harmonic generation are observed with the ring resonators. Because the large bandgap of GaP provides for low two-photon absorption at telecommunication wavelengths, the high-yield fabrication of GaP-on-insulator photonic devices enabled by this work is especially interesting for applications in nanophotonics, where high quality factors or low mode volumes can produce high electric field intensities. The large bandgap also enables integrated photonic devices operating at visible wavelengths.

  • Optomechanics with one-dimensional Gallium Phosphide photonic crystal cavities
    2017
    Co-Authors: Katharina Schneider, Yannick Baumgartner, Simon Honl, Pol Welter, Herwig Hahn, Lukas Czornomaz, Paul Seidler
    Abstract:

    We present the first investigation of optomechanics in an integrated one-dimensional Gallium Phosphide (GaP) photonic crystal cavity. The devices are fabricated with a newly developed process flow for integration of GaP devices on silicon dioxide (SiO2) involving direct wafer bonding of an epitaxial GaP/AlxGa1-xP/GaP heterostructure onto an oxidized silicon wafer. Device designs are transferred into the top GaP layer by inductively-coupled-plasma reactive ion etching and made freestanding by removal of the underlying SiO2. Finite-element simulations of the photonic crystal cavities predict optical quality factors greater than 106 at a design wavelength of 1550 nm and optomechanical coupling rates as high as 900 kHz for the mechanical breathing mode localized in the center of the photonic crystal cavity. The first fabricated devices exhibit optical quality factors as high as 6.5 × 104, and the mechanical breathing mode is found to have a vacuum coupling rate of 200 kHz at a frequency of 2.59 GHz. These results, combined with low two-photon absorption at telecommunication wavelengths and piezoelectric behavior, make GaP a promising material for the development of future nanophotonic devices in which optical and mechanical modes as well as high-frequency electrical signals interact.