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Yoshio Nishi - One of the best experts on this subject based on the ideXlab platform.

  • hfo 2 ti interface mediated Conductive Filament formation in rram an ab initio study
    IEEE Transactions on Electron Devices, 2018
    Co-Authors: Boubacar Traore, Blanka Magyarikope, Philippe Blaise, Benoit Sklenard, Elisa Vianello, Yoshio Nishi
    Abstract:

    We address the role of the Ti/HfO2 interface on the Conductive Filament (CF) formation within the context of oxide-based resistive random access memories (OxRRAMs). We investigate oxygen defects formation and diffusion at the interface through ab initio calculations. The calculated diffusion energy barriers compare well with the available experimental data. Through the interface region charge analysis and the associated energies with O defect formation and migration into Ti, our results support a probable CF growth from the interface region toward the electron injecting electrode, which acts as a cathode. Hence, for a Ti/HfO2-based OxRRAM supported by the calculation results, we present a pertinent CF growth model by considering its earliest stages, which is relevant for device modeling.

  • HfO2/Ti Interface Mediated Conductive Filament Formation in RRAM: An Ab Initio Study
    IEEE Transactions on Electron Devices, 2018
    Co-Authors: Boubacar Traore, Blanka Magyari-köpe, Philippe Blaise, Benoit Sklenard, Elisa Vianello, Yoshio Nishi
    Abstract:

    We address the role of the Ti/HfO2 interface on the Conductive Filament (CF) formation within the context of oxide-based resistive random access memories (OxRRAMs). We investigate oxygen defects formation and diffusion at the interface through ab initio calculations. The calculated diffusion energy barriers compare well with the available experimental data. Through the interface region charge analysis and the associated energies with O defect formation and migration into Ti, our results support a probable CF growth from the interface region toward the electron injecting electrode, which acts as a cathode. Hence, for a Ti/HfO2-based OxRRAM supported by the calculation results, we present a pertinent CF growth model by considering its earliest stages, which is relevant for device modeling.

  • HfO 2 /Ti Interface Mediated Conductive Filament Formation in RRAM: An Ab Initio Study
    IEEE Transactions on Electron Devices, 2018
    Co-Authors: Boubacar Traore, Blanka Magyari-köpe, Philippe Blaise, Benoit Sklenard, Elisa Vianello, Yoshio Nishi
    Abstract:

    We address the role of the Ti/HfO2 interface on the Conductive Filament (CF) formation within the context of oxide-based resistive random access memories (OxRRAMs). We investigate oxygen defects formation and diffusion at the interface through ab initio calculations. The calculated diffusion energy barriers compare well with the available experimental data. Through the interface region charge analysis and the associated energies with O defect formation and migration into Ti, our results support a probable CF growth from the interface region toward the electron injecting electrode, which acts as a cathode. Hence, for a Ti/HfO2-based OxRRAM supported by the calculation results, we present a pertinent CF growth model by considering its earliest stages, which is relevant for device modeling.

  • H-treatment impact on Conductive-Filament formation and stability in Ta2O5-based resistive-switching memory cells
    Journal of Applied Physics, 2015
    Co-Authors: Ludovic Goux, Blanka Magyari-köpe, Yoshio Nishi, Ja-yong Kim, Augusto Redolfi, Malgorzata Jurczak
    Abstract:

    In this article, we evidence the lower formation energy and improved stability of the Conductive Filament (CF) formed in TiN\Ta2O5\Ta resistive-switching memory cells treated in NH3 atmosphere at 400 °C. This annealing treatment results in (i) lower forming voltage, (ii) lower CF resistance, and (iii) longer retention lifetime of the oxygen-vacancy (Vo) chain constituting the CF. Atomistic insights into these processes are provided by ab initio calculations performed for hydrogen (H) species incorporated in non-stoichiometric Ta2O5 supercells: (i) Vo formation energy is reduced by the presence of H, (ii) Vo-chain CF conductivity is increased by Vo + OH complex formation, and (iii) Vo-chain retention is strengthened by the stable Vo + OH complex. As a result, efficient CF formation and excellent state stability are obtained after 15 days at 250 °C.

  • First-principles investigation of the Conductive Filament configuration in rutile TiO 2-x ReRAM
    MRS Proceedings, 2012
    Co-Authors: Liang Zhao, Seong-geon Park, Blanka Magyari-köpe, Yoshio Nishi
    Abstract:

    ABSTRACTThe interactions and ordering of oxygen vacancies in rutile TiO2 were thoroughly investigated by density functional calculations to search for atomic configurations of the Conductive Filament. As random isolated vacancies could not support the low-resistance state conduction in TiO2 ReRAM, vacancy ordering was introduced in [110] and [001] directions of the lattice to study the electronic structures. The calculation results revealed that a di-vacancy chain in [001] direction makes the electrons delocalized in that direction, which is identified as a possible configuration of the Conductive Filament. This low-resistance state can be effectively disrupted by moving oxygen vacancies out of the Filament to reach high-resistance states.

Ming Liu - One of the best experts on this subject based on the ideXlab platform.

  • Correlation analysis between the current fluctuation characteristics and the Conductive Filament morphology of HfO2-based memristor
    Applied Physics Letters, 2017
    Co-Authors: Kang-sheng Yin, Shibing Long, Meiyun Zhang, Long Cheng, Ya-xiong Zhou, Zhuo-rui Wang, Kan-hao Xue, Ming Liu
    Abstract:

    Memristors are attracting considerable interest for their prospective applications in nonvolatile memory, neuromorphic computing, and in-memory computing. However, the nature of resistance switching is still under debate, and current fluctuation in memristors is one of the critical concerns for stable performance. In this work, random telegraph noise (RTN) as the indication of current instabilities in distinct resistance states of the Pt/Ti/HfO2/W memristor is thoroughly investigated. Standard two-level digital-like RTN, multilevel current instabilities with non-correlation/correlation defects, and irreversible current transitions are observed and analyzed. The dependence of RTN on the resistance and read bias reveals that the current fluctuation depends strongly on the morphology and evolution of the Conductive Filament composed of oxygen vacancies. Our results link the current fluctuation behaviors to the evolution of the Conductive Filament and will guide continuous optimization of memristive devices.

  • Investigation on the Conductive Filament Growth Dynamics in Resistive Switching Memory via a Universal Monte Carlo Simulator
    Scientific Reports, 2017
    Co-Authors: Yu Li, Jiao Teng, Hangbing Lv, Shibing Long, Jordi Suñé, Enrique Miranda, Meiyun Zhang, Qi Liu, Ming Liu
    Abstract:

    In resistive random access memories, modeling Conductive Filament growing dynamics is important to understand the switching mechanism and variability. In this paper, a universal Monte Carlo simulator is developed based on a cell switching model and a tunneling-based transport model. Driven by external electric field, the growing process of the nanoscale Filament occurring in the gap region is actually dominated by cells’ Conductive/insulating switching, modeled through a phenomenological physics-based probability function. The electric transport through the partially formed CF is considered as current tunneling in the framework of the Quantum Point Contact model, and the potential barrier is modulated during cells’ evolution. To demonstrate the validity and universality of our simulator, various operation schemes are simulated, with the simulated I  −  V characteristics well explaining experimental observations. Furthermore, the statistical analyses of simulation results in terms of Weibull distribution and conductance evolution also nicely track previous experimental results. Representing a simulation scale that links atomic-scale simulations to compact modeling, our simulator has the advantage of being much faster comparing with other atomic-scale models. Meanwhile, our simulator shows good universality since it can be applied to various operation signals, and also to different electrodes and dielectric layers dominated by different switching mechanisms.

  • Resistive Switching Performance Improvement via Modulating Nanoscale Conductive Filament, Involving the Application of Two-Dimensional Layered Materials.
    Small (Weinheim an der Bergstrasse Germany), 2017
    Co-Authors: Shibing Long, Qi Liu, Ming Liu
    Abstract:

    Reversible chemical and structural changes induced by ionic motion and reaction in response to electrical stimuli leads to resistive switching effects in metal-insulator-metal structures. Filamentary switching based on the formation and rupture of nanoscale Conductive Filament has been applied in non-volatile memory and volatile selector devices with low power consumption and fast switching speeds. Before the mass production of resistive switching devices, great efforts are still required to enable stable and reliable switching performances. The Conductive Filament, a bridge of microscopic metal-insulator-metal structure and macroscopic resistance states, plays an irreplaceable part in resistive switching behavior, as unreliable performance often originates from unstable Filament behavior. In this Review, departing from the Filamentary switching mechanism and the existing issues, recent advances of the switching performance improvement through the Conductive Filament modulation are discussed, in the sequence of material modulation, device structure design and switching operation scheme optimization. In particular, two-dimensional (2D) nanomaterials with excellent properties including and beyond graphene, are discussed with emphasis on performance improvement by their active roles as the switching layer, insertion layer, thin electrode, patterned electrode, and edge electrode, etc.

  • anisotropic magnetoresistance of nano Conductive Filament in co hfo2 pt resistive switching memory
    Nanoscale Research Letters, 2017
    Co-Authors: Yang Liu, Jiao Teng, Shibing Long, Meiyun Zhang, Qi Liu, Qixun Guo, Ming Liu
    Abstract:

    Conductive bridge random access memory (CBRAM) has been extensively studied as a next-generation non-volatile memory. The Conductive Filament (CF) shows rich physical effects such as conductance quantization and magnetic effect. But so far, the study of Filaments is not very sufficient. In this work, Co/HfO2/Pt CBRAM device with magnetic CF was designed and fabricated. By electrical manipulation with a partial-RESET method, we controlled the size of ferromagnetic metal Filament. The resistance-temperature characteristics of the ON-state after various partial-RESET behaviors have been studied. Using two kinds of magnetic measurement methods, we measured the anisotropic magnetoresistance (AMR) of the CF at different temperatures to reflect the magnetic structure characteristics. By rotating the direction of the magnetic field and by sweeping the magnitude, we obtained the spatial direction as well as the easy-axis of the CF. The results indicate that the easy-axis of the CF is along the direction perpendicular to the top electrode plane. The maximum magnetoresistance was found to appear when the angle between the direction of magnetic field and that of the electric current in the CF is about 30°, and this angle varies slightly with temperature, indicating that the current is tilted.

  • justification and monte carlo simulation of microstructure evolution process of Conductive Filament in reset transition in cu hfo 2 pt rram
    International Symposium on the Physical and Failure Analysis of Integrated Circuits, 2015
    Co-Authors: Meiyun Zhang, Shibing Long, Qi Liu, Guoming Wang, Haitao Sun, Ming Liu
    Abstract:

    We proposed a new statistical evaluation method to justify the microstructure evolution process of Conductive Filament (CF) in the reset operation of resistive switching memory (RRAM) according to the dependence of the Weibull slope of reset parameters on the CF size. We demonstrated that in Cu/HfO 2 /Pt device the CF can be controlled to be ruptured abruptly, which is more advantageous to the reliable operation of RRAM since the intermediate states are avoided. A Monte Carlo (MC) simulator based on the thermal dissolution model is conducted to further prove our experimental results.

Seong-geon Park - One of the best experts on this subject based on the ideXlab platform.

  • First-principles investigation of the Conductive Filament configuration in rutile TiO 2-x ReRAM
    MRS Proceedings, 2012
    Co-Authors: Liang Zhao, Seong-geon Park, Blanka Magyari-köpe, Yoshio Nishi
    Abstract:

    ABSTRACTThe interactions and ordering of oxygen vacancies in rutile TiO2 were thoroughly investigated by density functional calculations to search for atomic configurations of the Conductive Filament. As random isolated vacancies could not support the low-resistance state conduction in TiO2 ReRAM, vacancy ordering was introduced in [110] and [001] directions of the lattice to study the electronic structures. The calculation results revealed that a di-vacancy chain in [001] direction makes the electrons delocalized in that direction, which is identified as a possible configuration of the Conductive Filament. This low-resistance state can be effectively disrupted by moving oxygen vacancies out of the Filament to reach high-resistance states.

  • impact of oxygen vacancy ordering on the formation of a Conductive Filament in hbox tio _ 2 for resistive switching memory
    IEEE Electron Device Letters, 2011
    Co-Authors: Seong-geon Park, Blanka Magyarikope, Yoshio Nishi
    Abstract:

    The electronic properties of rutile TiO2 with an ordered arrangement of oxygen vacancies show a transition from a resistive to Conductive oxide as a function of vacancy ordering. Vacancy ordering along two different directions [110] and [001], studied by the density functional theory, predicts that the geometries in which the vacancy-to-vacancy interaction is the strongest, within the nearest neighbor coordination, are thermodynamically favorable and of technological importance. The oxygen vacancies induce several occupied defect states of Ti 3d character, and according to our model, the vacancies are the mediators of electron conduction, while the Conductive Filament is formed by Ti ions. We propose that the formation of these types of Conductive Filament is intrinsically connected to the observed defect-assisted tunneling processes and oxide breakdown issues.

  • Impact of Oxygen Vacancy Ordering on the Formation of a Conductive Filament in $\hbox{TiO}_{2}$ for Resistive Switching Memory
    IEEE Electron Device Letters, 2011
    Co-Authors: Seong-geon Park, Blanka Magyari-köpe, Yoshio Nishi
    Abstract:

    The electronic properties of rutile TiO2 with an ordered arrangement of oxygen vacancies show a transition from a resistive to Conductive oxide as a function of vacancy ordering. Vacancy ordering along two different directions [110] and [001], studied by the density functional theory, predicts that the geometries in which the vacancy-to-vacancy interaction is the strongest, within the nearest neighbor coordination, are thermodynamically favorable and of technological importance. The oxygen vacancies induce several occupied defect states of Ti 3d character, and according to our model, the vacancies are the mediators of electron conduction, while the Conductive Filament is formed by Ti ions. We propose that the formation of these types of Conductive Filament is intrinsically connected to the observed defect-assisted tunneling processes and oxide breakdown issues.

Takeshi Takagi - One of the best experts on this subject based on the ideXlab platform.

Blanka Magyari-köpe - One of the best experts on this subject based on the ideXlab platform.

  • HfO2/Ti Interface Mediated Conductive Filament Formation in RRAM: An Ab Initio Study
    IEEE Transactions on Electron Devices, 2018
    Co-Authors: Boubacar Traore, Blanka Magyari-köpe, Philippe Blaise, Benoit Sklenard, Elisa Vianello, Yoshio Nishi
    Abstract:

    We address the role of the Ti/HfO2 interface on the Conductive Filament (CF) formation within the context of oxide-based resistive random access memories (OxRRAMs). We investigate oxygen defects formation and diffusion at the interface through ab initio calculations. The calculated diffusion energy barriers compare well with the available experimental data. Through the interface region charge analysis and the associated energies with O defect formation and migration into Ti, our results support a probable CF growth from the interface region toward the electron injecting electrode, which acts as a cathode. Hence, for a Ti/HfO2-based OxRRAM supported by the calculation results, we present a pertinent CF growth model by considering its earliest stages, which is relevant for device modeling.

  • HfO 2 /Ti Interface Mediated Conductive Filament Formation in RRAM: An Ab Initio Study
    IEEE Transactions on Electron Devices, 2018
    Co-Authors: Boubacar Traore, Blanka Magyari-köpe, Philippe Blaise, Benoit Sklenard, Elisa Vianello, Yoshio Nishi
    Abstract:

    We address the role of the Ti/HfO2 interface on the Conductive Filament (CF) formation within the context of oxide-based resistive random access memories (OxRRAMs). We investigate oxygen defects formation and diffusion at the interface through ab initio calculations. The calculated diffusion energy barriers compare well with the available experimental data. Through the interface region charge analysis and the associated energies with O defect formation and migration into Ti, our results support a probable CF growth from the interface region toward the electron injecting electrode, which acts as a cathode. Hence, for a Ti/HfO2-based OxRRAM supported by the calculation results, we present a pertinent CF growth model by considering its earliest stages, which is relevant for device modeling.

  • H-treatment impact on Conductive-Filament formation and stability in Ta2O5-based resistive-switching memory cells
    Journal of Applied Physics, 2015
    Co-Authors: Ludovic Goux, Blanka Magyari-köpe, Yoshio Nishi, Ja-yong Kim, Augusto Redolfi, Malgorzata Jurczak
    Abstract:

    In this article, we evidence the lower formation energy and improved stability of the Conductive Filament (CF) formed in TiN\Ta2O5\Ta resistive-switching memory cells treated in NH3 atmosphere at 400 °C. This annealing treatment results in (i) lower forming voltage, (ii) lower CF resistance, and (iii) longer retention lifetime of the oxygen-vacancy (Vo) chain constituting the CF. Atomistic insights into these processes are provided by ab initio calculations performed for hydrogen (H) species incorporated in non-stoichiometric Ta2O5 supercells: (i) Vo formation energy is reduced by the presence of H, (ii) Vo-chain CF conductivity is increased by Vo + OH complex formation, and (iii) Vo-chain retention is strengthened by the stable Vo + OH complex. As a result, efficient CF formation and excellent state stability are obtained after 15 days at 250 °C.

  • First-principles investigation of the Conductive Filament configuration in rutile TiO 2-x ReRAM
    MRS Proceedings, 2012
    Co-Authors: Liang Zhao, Seong-geon Park, Blanka Magyari-köpe, Yoshio Nishi
    Abstract:

    ABSTRACTThe interactions and ordering of oxygen vacancies in rutile TiO2 were thoroughly investigated by density functional calculations to search for atomic configurations of the Conductive Filament. As random isolated vacancies could not support the low-resistance state conduction in TiO2 ReRAM, vacancy ordering was introduced in [110] and [001] directions of the lattice to study the electronic structures. The calculation results revealed that a di-vacancy chain in [001] direction makes the electrons delocalized in that direction, which is identified as a possible configuration of the Conductive Filament. This low-resistance state can be effectively disrupted by moving oxygen vacancies out of the Filament to reach high-resistance states.

  • Impact of Oxygen Vacancy Ordering on the Formation of a Conductive Filament in $\hbox{TiO}_{2}$ for Resistive Switching Memory
    IEEE Electron Device Letters, 2011
    Co-Authors: Seong-geon Park, Blanka Magyari-köpe, Yoshio Nishi
    Abstract:

    The electronic properties of rutile TiO2 with an ordered arrangement of oxygen vacancies show a transition from a resistive to Conductive oxide as a function of vacancy ordering. Vacancy ordering along two different directions [110] and [001], studied by the density functional theory, predicts that the geometries in which the vacancy-to-vacancy interaction is the strongest, within the nearest neighbor coordination, are thermodynamically favorable and of technological importance. The oxygen vacancies induce several occupied defect states of Ti 3d character, and according to our model, the vacancies are the mediators of electron conduction, while the Conductive Filament is formed by Ti ions. We propose that the formation of these types of Conductive Filament is intrinsically connected to the observed defect-assisted tunneling processes and oxide breakdown issues.