The Experts below are selected from a list of 360 Experts worldwide ranked by ideXlab platform

Atsuhiro Osuka - One of the best experts on this subject based on the ideXlab platform.

Naoki Komatsu - One of the best experts on this subject based on the ideXlab platform.

  • Simultaneous Discrimination of Diameter, Handedness, and Metallicity of Single-Walled Carbon Nanotubes with Chiral Diporphyrin Nanocalipers
    2016
    Co-Authors: Gang Liu, Takahide Kimura, Feng Wang, Yukie Saito, Ajoy K. Bauri, Songpol Chaunchaiyakul, Yuji Kuwahara, Naoki Komatsu
    Abstract:

    We have been developing the methodology to discriminate the handedness and diameter of single-walled carbon nanotubes (SWNTs) through molecular recognition using chiral Diporphyrin nanotweezers. Although relatively small diameters of SWNTs (1.0 nm. In this context, we designed chiral Diporphyrin with a much larger cavity, namely, “nanocalipers”. The feature of the newly designed host molecule is: (1) long spacer with more than 1.4 nm consisting of three aromatic moieties; (2) nearly parallel orientation of the two porphyrins; (3) restricted conformation by biaryl linkages of the porphyrin–carbazole and carbazole–anthracene; (4) strong interaction of two porphyrins and anthracene with the surface of a SWNT through π–π stacking; and (5) stereogenic centers at the periphery of porphyrins discriminating helicity of SWNTs. As expected, we obtained optically active SWNTs with >1.0 nm in diameter and, unexpectedly, enriched metallic SWNTs over semiconducting ones. The optically active metallic SWNTs are identified for the first time, in addition to the optically active semiconducting SWNTs with such large diameters. The nanocalipers are found to recognize the diameter, handedness, and metallicity of SWNTs simultaneously

  • Structural discrimination of double-walled carbon nanotubes by chiral Diporphyrin nanocalipers
    Journal of Materials Chemistry A, 2014
    Co-Authors: Gang Liu, Takahide Kimura, Yukie Saito, Daisuke Nishio-hamane, Ajoy K. Bauri, Emmanuel Flahaut, Naoki Komatsu
    Abstract:

    In this contribution, we demonstrate the separation of double-walled carbon nanotubes (DWNTs) by host–guest methodology. New chiral Diporphyrin nanocalipers with a longer spacer ([similar]1.9 nm) consisting of carbazole–pyrene–carbazole are rationally designed as a host on the basis of the previous chiral Diporphyrin nanocalipers with carbazole–anthracene–carbazole spacer ([similar]1.4 nm). The chiral nanocalipers are found to recognize the diameter of DWNTs to make diameter distribution much narrower. In addition, the extracted carbon nanotubes (CNTs) exhibited circular dichroism (CD) after removal of the chiral nanocalipers and dissolution in water in the presence of achiral surfactant.

  • simultaneous discrimination of diameter handedness and metallicity of single walled carbon nanotubes with chiral Diporphyrin nanocalipers
    Journal of the American Chemical Society, 2013
    Co-Authors: Gang Liu, Takahide Kimura, Feng Wang, Yukie Saito, Ajoy Kumar Bauri, Songpol Chaunchaiyakul, Yuji Kuwahara, Naoki Komatsu
    Abstract:

    We have been developing the methodology to discriminate the handedness and diameter of single-walled carbon nanotubes (SWNTs) through molecular recognition using chiral Diporphyrin nanotweezers. Although relatively small diameters of SWNTs ( 1.0 nm. In this context, we designed chiral Diporphyrin with a much larger cavity, namely, "nanocalipers". The feature of the newly designed host molecule is: (1) long spacer with more than 1.4 nm consisting of three aromatic moieties; (2) nearly parallel orientation of the two porphyrins; (3) restricted conformation by biaryl linkages of the porphyrin-carbazole and carbazole-anthracene; (4) strong interaction of two porphyrins and anthracene with the surface of a SWNT through π-π stacking; and (5) stereogenic centers at the periphery of porphyrins discriminating helicity of SWNTs. As expected, we obtained optically active SWNTs with >1.0 nm in diameter and, unexpectedly, enriched metallic SWNTs over semiconducting ones. The optically active metallic SWNTs are identified for the first time, in addition to the optically active semiconducting SWNTs with such large diameters. The nanocalipers are found to recognize the diameter, handedness, and metallicity of SWNTs simultaneously.

  • preferential extraction of left or right handed single walled carbon nanotubes by use of chiral Diporphyrin nanotweezers
    Organic and Biomolecular Chemistry, 2012
    Co-Authors: Gang Liu, Xiaobin Peng, Shuji Aonuma, Takahide Kimura, Feng Wang, Tatsuki Yasumitsu, Li Zhao, Ajoy Kumar Bauri, Naoki Komatsu
    Abstract:

    Handedness- and diameter-based separation of single-walled carbon nanotubes was achieved through preferential extraction of 76-CoMoCAT with 2,6-pyridylene-bridged chiral Diporphyrin nanotweezers.

  • improved selectivity in discriminating handedness and diameter of single walled carbon nanotubes with n substituted 3 6 carbazolylene bridged chiral Diporphyrin nanotweezers
    Nanoscale, 2011
    Co-Authors: Feng Wang, Takahide Kimura, Kazunari Matsuda, A Mustafizur F M Rahman, Naoki Komatsu
    Abstract:

    Chiral Diporphyrin nanotweezers 1 consisting of two chiral porphyrins with N-substituted 3,6-carbazolylene in between have been studied for the separation of single-walled carbon nanotubes (SWNTs). As compared to the analogous nanotweezers 2 without an N-substitutent, nanotweezers 1 with the N-octylcarbazolylene spacer exhibit much higher extraction ability and better selectivity for SWNTs. A narrower diameter range of SWNTs, from 0.88 to 0.92 nm, was selectively extracted with nanotweezers 1. In addition, only (7,6)-SWNTs of 0.90 nm diameter were optically enriched through extraction with 1, while SWNTs extracted with 2 showed lower optical purity of (7,6)-SWNTs. These enhanced extraction and discrimination abilities of 1 can be attributed to the formation of a more stable SWNT complex of 1 than of 2 in methanol.

Xiaobin Peng - One of the best experts on this subject based on the ideXlab platform.

Takahide Kimura - One of the best experts on this subject based on the ideXlab platform.

  • Simultaneous Discrimination of Diameter, Handedness, and Metallicity of Single-Walled Carbon Nanotubes with Chiral Diporphyrin Nanocalipers
    2016
    Co-Authors: Gang Liu, Takahide Kimura, Feng Wang, Yukie Saito, Ajoy K. Bauri, Songpol Chaunchaiyakul, Yuji Kuwahara, Naoki Komatsu
    Abstract:

    We have been developing the methodology to discriminate the handedness and diameter of single-walled carbon nanotubes (SWNTs) through molecular recognition using chiral Diporphyrin nanotweezers. Although relatively small diameters of SWNTs (1.0 nm. In this context, we designed chiral Diporphyrin with a much larger cavity, namely, “nanocalipers”. The feature of the newly designed host molecule is: (1) long spacer with more than 1.4 nm consisting of three aromatic moieties; (2) nearly parallel orientation of the two porphyrins; (3) restricted conformation by biaryl linkages of the porphyrin–carbazole and carbazole–anthracene; (4) strong interaction of two porphyrins and anthracene with the surface of a SWNT through π–π stacking; and (5) stereogenic centers at the periphery of porphyrins discriminating helicity of SWNTs. As expected, we obtained optically active SWNTs with >1.0 nm in diameter and, unexpectedly, enriched metallic SWNTs over semiconducting ones. The optically active metallic SWNTs are identified for the first time, in addition to the optically active semiconducting SWNTs with such large diameters. The nanocalipers are found to recognize the diameter, handedness, and metallicity of SWNTs simultaneously

  • Structural discrimination of double-walled carbon nanotubes by chiral Diporphyrin nanocalipers
    Journal of Materials Chemistry A, 2014
    Co-Authors: Gang Liu, Takahide Kimura, Yukie Saito, Daisuke Nishio-hamane, Ajoy K. Bauri, Emmanuel Flahaut, Naoki Komatsu
    Abstract:

    In this contribution, we demonstrate the separation of double-walled carbon nanotubes (DWNTs) by host–guest methodology. New chiral Diporphyrin nanocalipers with a longer spacer ([similar]1.9 nm) consisting of carbazole–pyrene–carbazole are rationally designed as a host on the basis of the previous chiral Diporphyrin nanocalipers with carbazole–anthracene–carbazole spacer ([similar]1.4 nm). The chiral nanocalipers are found to recognize the diameter of DWNTs to make diameter distribution much narrower. In addition, the extracted carbon nanotubes (CNTs) exhibited circular dichroism (CD) after removal of the chiral nanocalipers and dissolution in water in the presence of achiral surfactant.

  • simultaneous discrimination of diameter handedness and metallicity of single walled carbon nanotubes with chiral Diporphyrin nanocalipers
    Journal of the American Chemical Society, 2013
    Co-Authors: Gang Liu, Takahide Kimura, Feng Wang, Yukie Saito, Ajoy Kumar Bauri, Songpol Chaunchaiyakul, Yuji Kuwahara, Naoki Komatsu
    Abstract:

    We have been developing the methodology to discriminate the handedness and diameter of single-walled carbon nanotubes (SWNTs) through molecular recognition using chiral Diporphyrin nanotweezers. Although relatively small diameters of SWNTs ( 1.0 nm. In this context, we designed chiral Diporphyrin with a much larger cavity, namely, "nanocalipers". The feature of the newly designed host molecule is: (1) long spacer with more than 1.4 nm consisting of three aromatic moieties; (2) nearly parallel orientation of the two porphyrins; (3) restricted conformation by biaryl linkages of the porphyrin-carbazole and carbazole-anthracene; (4) strong interaction of two porphyrins and anthracene with the surface of a SWNT through π-π stacking; and (5) stereogenic centers at the periphery of porphyrins discriminating helicity of SWNTs. As expected, we obtained optically active SWNTs with >1.0 nm in diameter and, unexpectedly, enriched metallic SWNTs over semiconducting ones. The optically active metallic SWNTs are identified for the first time, in addition to the optically active semiconducting SWNTs with such large diameters. The nanocalipers are found to recognize the diameter, handedness, and metallicity of SWNTs simultaneously.

  • preferential extraction of left or right handed single walled carbon nanotubes by use of chiral Diporphyrin nanotweezers
    Organic and Biomolecular Chemistry, 2012
    Co-Authors: Gang Liu, Xiaobin Peng, Shuji Aonuma, Takahide Kimura, Feng Wang, Tatsuki Yasumitsu, Li Zhao, Ajoy Kumar Bauri, Naoki Komatsu
    Abstract:

    Handedness- and diameter-based separation of single-walled carbon nanotubes was achieved through preferential extraction of 76-CoMoCAT with 2,6-pyridylene-bridged chiral Diporphyrin nanotweezers.

  • improved selectivity in discriminating handedness and diameter of single walled carbon nanotubes with n substituted 3 6 carbazolylene bridged chiral Diporphyrin nanotweezers
    Nanoscale, 2011
    Co-Authors: Feng Wang, Takahide Kimura, Kazunari Matsuda, A Mustafizur F M Rahman, Naoki Komatsu
    Abstract:

    Chiral Diporphyrin nanotweezers 1 consisting of two chiral porphyrins with N-substituted 3,6-carbazolylene in between have been studied for the separation of single-walled carbon nanotubes (SWNTs). As compared to the analogous nanotweezers 2 without an N-substitutent, nanotweezers 1 with the N-octylcarbazolylene spacer exhibit much higher extraction ability and better selectivity for SWNTs. A narrower diameter range of SWNTs, from 0.88 to 0.92 nm, was selectively extracted with nanotweezers 1. In addition, only (7,6)-SWNTs of 0.90 nm diameter were optically enriched through extraction with 1, while SWNTs extracted with 2 showed lower optical purity of (7,6)-SWNTs. These enhanced extraction and discrimination abilities of 1 can be attributed to the formation of a more stable SWNT complex of 1 than of 2 in methanol.

Feng Wang - One of the best experts on this subject based on the ideXlab platform.

  • Simultaneous Discrimination of Diameter, Handedness, and Metallicity of Single-Walled Carbon Nanotubes with Chiral Diporphyrin Nanocalipers
    2016
    Co-Authors: Gang Liu, Takahide Kimura, Feng Wang, Yukie Saito, Ajoy K. Bauri, Songpol Chaunchaiyakul, Yuji Kuwahara, Naoki Komatsu
    Abstract:

    We have been developing the methodology to discriminate the handedness and diameter of single-walled carbon nanotubes (SWNTs) through molecular recognition using chiral Diporphyrin nanotweezers. Although relatively small diameters of SWNTs (1.0 nm. In this context, we designed chiral Diporphyrin with a much larger cavity, namely, “nanocalipers”. The feature of the newly designed host molecule is: (1) long spacer with more than 1.4 nm consisting of three aromatic moieties; (2) nearly parallel orientation of the two porphyrins; (3) restricted conformation by biaryl linkages of the porphyrin–carbazole and carbazole–anthracene; (4) strong interaction of two porphyrins and anthracene with the surface of a SWNT through π–π stacking; and (5) stereogenic centers at the periphery of porphyrins discriminating helicity of SWNTs. As expected, we obtained optically active SWNTs with >1.0 nm in diameter and, unexpectedly, enriched metallic SWNTs over semiconducting ones. The optically active metallic SWNTs are identified for the first time, in addition to the optically active semiconducting SWNTs with such large diameters. The nanocalipers are found to recognize the diameter, handedness, and metallicity of SWNTs simultaneously

  • simultaneous discrimination of diameter handedness and metallicity of single walled carbon nanotubes with chiral Diporphyrin nanocalipers
    Journal of the American Chemical Society, 2013
    Co-Authors: Gang Liu, Takahide Kimura, Feng Wang, Yukie Saito, Ajoy Kumar Bauri, Songpol Chaunchaiyakul, Yuji Kuwahara, Naoki Komatsu
    Abstract:

    We have been developing the methodology to discriminate the handedness and diameter of single-walled carbon nanotubes (SWNTs) through molecular recognition using chiral Diporphyrin nanotweezers. Although relatively small diameters of SWNTs ( 1.0 nm. In this context, we designed chiral Diporphyrin with a much larger cavity, namely, "nanocalipers". The feature of the newly designed host molecule is: (1) long spacer with more than 1.4 nm consisting of three aromatic moieties; (2) nearly parallel orientation of the two porphyrins; (3) restricted conformation by biaryl linkages of the porphyrin-carbazole and carbazole-anthracene; (4) strong interaction of two porphyrins and anthracene with the surface of a SWNT through π-π stacking; and (5) stereogenic centers at the periphery of porphyrins discriminating helicity of SWNTs. As expected, we obtained optically active SWNTs with >1.0 nm in diameter and, unexpectedly, enriched metallic SWNTs over semiconducting ones. The optically active metallic SWNTs are identified for the first time, in addition to the optically active semiconducting SWNTs with such large diameters. The nanocalipers are found to recognize the diameter, handedness, and metallicity of SWNTs simultaneously.

  • preferential extraction of left or right handed single walled carbon nanotubes by use of chiral Diporphyrin nanotweezers
    Organic and Biomolecular Chemistry, 2012
    Co-Authors: Gang Liu, Xiaobin Peng, Shuji Aonuma, Takahide Kimura, Feng Wang, Tatsuki Yasumitsu, Li Zhao, Ajoy Kumar Bauri, Naoki Komatsu
    Abstract:

    Handedness- and diameter-based separation of single-walled carbon nanotubes was achieved through preferential extraction of 76-CoMoCAT with 2,6-pyridylene-bridged chiral Diporphyrin nanotweezers.

  • improved selectivity in discriminating handedness and diameter of single walled carbon nanotubes with n substituted 3 6 carbazolylene bridged chiral Diporphyrin nanotweezers
    Nanoscale, 2011
    Co-Authors: Feng Wang, Takahide Kimura, Kazunari Matsuda, A Mustafizur F M Rahman, Naoki Komatsu
    Abstract:

    Chiral Diporphyrin nanotweezers 1 consisting of two chiral porphyrins with N-substituted 3,6-carbazolylene in between have been studied for the separation of single-walled carbon nanotubes (SWNTs). As compared to the analogous nanotweezers 2 without an N-substitutent, nanotweezers 1 with the N-octylcarbazolylene spacer exhibit much higher extraction ability and better selectivity for SWNTs. A narrower diameter range of SWNTs, from 0.88 to 0.92 nm, was selectively extracted with nanotweezers 1. In addition, only (7,6)-SWNTs of 0.90 nm diameter were optically enriched through extraction with 1, while SWNTs extracted with 2 showed lower optical purity of (7,6)-SWNTs. These enhanced extraction and discrimination abilities of 1 can be attributed to the formation of a more stable SWNT complex of 1 than of 2 in methanol.

  • optical resolution of single walled carbon nanotubes through molecular recognition with chiral Diporphyrin nanotweezers
    ChemInform, 2011
    Co-Authors: Xiaobin Peng, Feng Wang, A Mustafizur F M Rahman, Ajoy Kumar Bauri, Naoki Komatsu
    Abstract:

    Single-walled carbon nanotubes (SWNTs) have either chiral or achiral form, and synthesized chiral SWNTs include both left- and right-handed structures in equal amounts. Recently, a racemic mixture ...