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T. Goto - One of the best experts on this subject based on the ideXlab platform.

  • Giant magnetocaloric effect in itinerant-electron metamagnets
    Physica B-condensed Matter, 2004
    Co-Authors: H Yamada, T. Goto
    Abstract:

    Abstract Based on the theory of the itinerant-electron Metamagnetism, an isothermal magnetic entropy change is discussed for 3d transition metal compounds. The magnetic entropy change depends not only on the magnetization jump at the Curie temperature, but also on the temperature dependence of the critical field of the metamagnetic transition. The isothermal magnetic entropy changes for Co(S,Se) 2 , Lu(Co,Al) 2 and Lu(Co,Ga) 2 are estimated and compared with those observed for MnFe(P,As) and La(Fe,Si) 13 .

  • Physics of anisotropic itinerant 5f-electron Metamagnetism in UCo1−xTxAl (T=Fe, Ni)
    Journal of Magnetism and Magnetic Materials, 2004
    Co-Authors: N.v. Mushnikov, T. Goto, H. Yamada, Alexander V. Andreev, Vladimír Sechovský
    Abstract:

    Abstract UCoAl is an itinerant 5f-electron metamagnet with a strong uniaxial anisotropy. We studied the magnetization of the UCo 1− x T x Al (T=Fe, Ni) single crystals as a function of magnetic field (0–9 T), temperature (1.5–40 K) and external pressure (0–1.2 GPa). The Ni substitution for Co yields an increase of the critical field of Metamagnetism. Contrary, just 2% substitution of Fe for Co in UCoAl stabilizes ferromagnetic ground state, while the reentrant Metamagnetism is observed in substitution-induced ferromagnets under pressure. Experimental data have been analyzed within the theory of itinerant electron Metamagnetism considering anisotropic thermal fluctuations of magnetic moment.

  • decoupling of the magnetic ordering of the rare earth and the co sublattice in er 1 x y x co 2 compounds driven by substitution or pressure
    Physical Review B, 2000
    Co-Authors: R Hauser, A. S. Markosyan, K. Kamishima, E. Bauer, E Gratz, H Muller, M Rotter, H Michor, G Hilscher, T. Goto
    Abstract:

    The thermodynamic and transport properties of the ${\mathrm{Er}}_{1\ensuremath{-}x}{\mathrm{Y}}_{x}{\mathrm{Co}}_{2}$ system were studied in the concentration range $0.0l~xl~1.0.$ In this system, the first-order magnetic phase transition observed in ${\mathrm{ErCo}}_{2}$ at ${T}_{\mathrm{C}}=32$ K is related to the itinerant electron Metamagnetism of the d subsystem (Co sublattice) driven by the onset of magnetic ordering within the Er sublattice. By employing magnetic, specific heat, thermal expansion, and resistivity measurements we show that in a limited concentration range ${x}_{{\mathrm{cr}}^{\ensuremath{'}}}lxl{x}_{\mathrm{cr}}$ and pressure ${P}_{{\mathrm{cr}}^{\ensuremath{'}}}lPl{P}_{\mathrm{cr}}$ the itinerant Co sublattice orders magnetically at ${T}_{\mathrm{C}}^{\mathrm{Co}},$ which is lower than ${T}_{\mathrm{C}}^{R}$ of the Er sublattice. This is referred either to a weakening of the effective molecular field acting on the Co sites owing to the yttrium subsititution or to a pressure-driven increase of the critical field necessary to induce a magnetic moment on the Co sites. On further increasing the yttrium concentration or the pressure only the Er sublattice exhibits long-range order. The theoretical calculations within the molecular field approximation are in agreement with the experimental magnetic x-$T$ phase diagram of the ${\mathrm{Er}}_{1\ensuremath{-}x}{\mathrm{Y}}_{x}{\mathrm{Co}}_{2}$ system and confirm the effect of a separate ordering of the magnetic sublattices with reasonable parameters used for the intrasublattice Er-Er and intersublattice Er-Co exchange interactions. A field-induced collapse of the Co moment, inverse itinerant electron Metamagnetism, is well observable by magnetoresistance measurements at appropriate values of concentration and external pressure. The existence of itinerant electron Metamagnetism in the Co sublattice is found to be limited in temperature by ${T}_{0},$ a characteristic temperature which is sensitive to substitution and pressure.

  • Effects of external pressure on the 5f-band Metamagnetism in UCoAl
    Physical Review B, 1997
    Co-Authors: Alexander V. Andreev, T. Goto, M.i. Bartashevich, K. Kamishima, Ladislav Havela, Vladimír Sechovský
    Abstract:

    UCoAl exhibits below 16 K anisotropic 5f-band Metamagnetism induced by magnetic fields as low as \ensuremath{\sim}1 T applied along the c axis of the hexagonal structure. No metamagnetic transition is observed in fields up to 40 T applied within the basal plane. The critical field of the metamagnetic transition ${\mathrm{B}}_{\mathrm{c}}$ is composition dependent within the homogeneity range. The metamagnetic transition is found to be very sensitive to external pressure. The value of ${\mathrm{B}}_{\mathrm{c}}$ increases with the rate ${\mathrm{dB}}_{\mathrm{c}}$ /dp=0.27 T/kbar, whereas the magnetization gained through the transition becomes reduced. The critical pressure of 24 kbar (corresponding to \ensuremath{\sim}2% volume contraction) for disappearance of Metamagnetism in UCoAl has been estimated. Relations of UCoAl to 3d-band metamagnets are discussed.

  • 5f-band Metamagnetism in UCoAl
    Physica B-condensed Matter, 1997
    Co-Authors: Ladislav Havela, T. Goto, Alexander V. Andreev, Vladimír Sechovský, M.i. Bartashevich, I.k Kozlovskaya, K. Prokes, Pavel Javorský, K. Kamishima
    Abstract:

    UCoAl is a 5f-band metamagnet characterized by a very low critical field Bc ≈ 0.8 T, which induces magnetization of 0.3 μB/f.u. by a distinct transition. Bc increases with increasing temperature with the rate consistent with the reduced γ-coefficient in the high-field state. Bc-values are also sensitive to stoichiometry and external pressure.

R. S. Perry - One of the best experts on this subject based on the ideXlab platform.

Vladimír Sechovský - One of the best experts on this subject based on the ideXlab platform.

  • Transition from Ferromagnetism to Metamagnetism under Pressure in a U0.94Y0.06CoAl Single Crystal
    Journal of the Physical Society of Japan, 2007
    Co-Authors: Alexander V. Andreev, N.v. Mushnikov, Vladimír Sechovský, Keiichi Koyama, Yoshinobu Shiokawa, Isamu Satoh, Kazuo Watanabe
    Abstract:

    Substitution of Y for U in the itinerant 5f-electron metamagnet UCoAl transforms the system to a ferromagnetic ground state. Application of external hydrostatic pressure above 0.3 GPa suppresses the ferromagnetism and restores the “UCoAl-type” Metamagnetism. However, the metamagnetic transition becomes of the second-order type instead of the first-order one for the parent UCoAl.

  • Physics of anisotropic itinerant 5f-electron Metamagnetism in UCo1−xTxAl (T=Fe, Ni)
    Journal of Magnetism and Magnetic Materials, 2004
    Co-Authors: N.v. Mushnikov, T. Goto, H. Yamada, Alexander V. Andreev, Vladimír Sechovský
    Abstract:

    Abstract UCoAl is an itinerant 5f-electron metamagnet with a strong uniaxial anisotropy. We studied the magnetization of the UCo 1− x T x Al (T=Fe, Ni) single crystals as a function of magnetic field (0–9 T), temperature (1.5–40 K) and external pressure (0–1.2 GPa). The Ni substitution for Co yields an increase of the critical field of Metamagnetism. Contrary, just 2% substitution of Fe for Co in UCoAl stabilizes ferromagnetic ground state, while the reentrant Metamagnetism is observed in substitution-induced ferromagnets under pressure. Experimental data have been analyzed within the theory of itinerant electron Metamagnetism considering anisotropic thermal fluctuations of magnetic moment.

  • Metamagnetism of UCoAl under high pressure
    Physica B-condensed Matter, 2000
    Co-Authors: Tsuneaki Goto, N.v. Mushnikov, Alexander V. Andreev, H Yamada, Vladimír Sechovský
    Abstract:

    Abstract The susceptibility and magnetization of metamagnetic UCoAl were measured under high pressures up to 1.2 GPa. The metamagnetic behavior under high pressure is very similar to that of a typical 3d itinerant metamagnet.

  • Effects of external pressure on the 5f-band Metamagnetism in UCoAl
    Physical Review B, 1997
    Co-Authors: Alexander V. Andreev, T. Goto, M.i. Bartashevich, K. Kamishima, Ladislav Havela, Vladimír Sechovský
    Abstract:

    UCoAl exhibits below 16 K anisotropic 5f-band Metamagnetism induced by magnetic fields as low as \ensuremath{\sim}1 T applied along the c axis of the hexagonal structure. No metamagnetic transition is observed in fields up to 40 T applied within the basal plane. The critical field of the metamagnetic transition ${\mathrm{B}}_{\mathrm{c}}$ is composition dependent within the homogeneity range. The metamagnetic transition is found to be very sensitive to external pressure. The value of ${\mathrm{B}}_{\mathrm{c}}$ increases with the rate ${\mathrm{dB}}_{\mathrm{c}}$ /dp=0.27 T/kbar, whereas the magnetization gained through the transition becomes reduced. The critical pressure of 24 kbar (corresponding to \ensuremath{\sim}2% volume contraction) for disappearance of Metamagnetism in UCoAl has been estimated. Relations of UCoAl to 3d-band metamagnets are discussed.

  • 5f-band Metamagnetism in UCoAl
    Physica B-condensed Matter, 1997
    Co-Authors: Ladislav Havela, T. Goto, Alexander V. Andreev, Vladimír Sechovský, M.i. Bartashevich, I.k Kozlovskaya, K. Prokes, Pavel Javorský, K. Kamishima
    Abstract:

    UCoAl is a 5f-band metamagnet characterized by a very low critical field Bc ≈ 0.8 T, which induces magnetization of 0.3 μB/f.u. by a distinct transition. Bc increases with increasing temperature with the rate consistent with the reduced γ-coefficient in the high-field state. Bc-values are also sensitive to stoichiometry and external pressure.

Chang Seop Hong - One of the best experts on this subject based on the ideXlab platform.

Alexander V. Andreev - One of the best experts on this subject based on the ideXlab platform.

  • Transition from Ferromagnetism to Metamagnetism under Pressure in a U0.94Y0.06CoAl Single Crystal
    Journal of the Physical Society of Japan, 2007
    Co-Authors: Alexander V. Andreev, N.v. Mushnikov, Vladimír Sechovský, Keiichi Koyama, Yoshinobu Shiokawa, Isamu Satoh, Kazuo Watanabe
    Abstract:

    Substitution of Y for U in the itinerant 5f-electron metamagnet UCoAl transforms the system to a ferromagnetic ground state. Application of external hydrostatic pressure above 0.3 GPa suppresses the ferromagnetism and restores the “UCoAl-type” Metamagnetism. However, the metamagnetic transition becomes of the second-order type instead of the first-order one for the parent UCoAl.

  • Physics of anisotropic itinerant 5f-electron Metamagnetism in UCo1−xTxAl (T=Fe, Ni)
    Journal of Magnetism and Magnetic Materials, 2004
    Co-Authors: N.v. Mushnikov, T. Goto, H. Yamada, Alexander V. Andreev, Vladimír Sechovský
    Abstract:

    Abstract UCoAl is an itinerant 5f-electron metamagnet with a strong uniaxial anisotropy. We studied the magnetization of the UCo 1− x T x Al (T=Fe, Ni) single crystals as a function of magnetic field (0–9 T), temperature (1.5–40 K) and external pressure (0–1.2 GPa). The Ni substitution for Co yields an increase of the critical field of Metamagnetism. Contrary, just 2% substitution of Fe for Co in UCoAl stabilizes ferromagnetic ground state, while the reentrant Metamagnetism is observed in substitution-induced ferromagnets under pressure. Experimental data have been analyzed within the theory of itinerant electron Metamagnetism considering anisotropic thermal fluctuations of magnetic moment.

  • Metamagnetism of UCoAl under high pressure
    Physica B-condensed Matter, 2000
    Co-Authors: Tsuneaki Goto, N.v. Mushnikov, Alexander V. Andreev, H Yamada, Vladimír Sechovský
    Abstract:

    Abstract The susceptibility and magnetization of metamagnetic UCoAl were measured under high pressures up to 1.2 GPa. The metamagnetic behavior under high pressure is very similar to that of a typical 3d itinerant metamagnet.

  • Effects of external pressure on the 5f-band Metamagnetism in UCoAl
    Physical Review B, 1997
    Co-Authors: Alexander V. Andreev, T. Goto, M.i. Bartashevich, K. Kamishima, Ladislav Havela, Vladimír Sechovský
    Abstract:

    UCoAl exhibits below 16 K anisotropic 5f-band Metamagnetism induced by magnetic fields as low as \ensuremath{\sim}1 T applied along the c axis of the hexagonal structure. No metamagnetic transition is observed in fields up to 40 T applied within the basal plane. The critical field of the metamagnetic transition ${\mathrm{B}}_{\mathrm{c}}$ is composition dependent within the homogeneity range. The metamagnetic transition is found to be very sensitive to external pressure. The value of ${\mathrm{B}}_{\mathrm{c}}$ increases with the rate ${\mathrm{dB}}_{\mathrm{c}}$ /dp=0.27 T/kbar, whereas the magnetization gained through the transition becomes reduced. The critical pressure of 24 kbar (corresponding to \ensuremath{\sim}2% volume contraction) for disappearance of Metamagnetism in UCoAl has been estimated. Relations of UCoAl to 3d-band metamagnets are discussed.

  • 5f-band Metamagnetism in UCoAl
    Physica B-condensed Matter, 1997
    Co-Authors: Ladislav Havela, T. Goto, Alexander V. Andreev, Vladimír Sechovský, M.i. Bartashevich, I.k Kozlovskaya, K. Prokes, Pavel Javorský, K. Kamishima
    Abstract:

    UCoAl is a 5f-band metamagnet characterized by a very low critical field Bc ≈ 0.8 T, which induces magnetization of 0.3 μB/f.u. by a distinct transition. Bc increases with increasing temperature with the rate consistent with the reduced γ-coefficient in the high-field state. Bc-values are also sensitive to stoichiometry and external pressure.