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  • Rethink about electrolyte: Potassium Fluoride as a promising additive to an electrolyte for the water oxidation by a nanolayered Mn oxide
    International Journal of Hydrogen Energy, 2017
    Co-Authors: Mohammad Mahdi Najafpour, Seyedeh Maedeh Hosseini, Mohadeseh Zarei Ghobadi, Parvin Rafighi, Robabeh Bagheri, Keun Hwa Chae, Somayeh Mehrabani, Zhenlun Song
    Abstract:

    Abstract Water oxidation is a bottleneck of the hydrogen production through the water-splitting reaction. Herein, the promising role of Fluoride on the water-oxidizing activity of a nanolayered Mn oxide under the electrochemical condition is reported. The experiments show the increase of the water-oxidizing activity of the nanolayered Mn oxide under an electro-water oxidation circumstance in the presence of Potassium Fluoride as a promising additive to an electrolyte. As a result, the required overpotential is decreased and the yield of oxygen evolution raised in the water-oxidation reaction.

  • treated nanolayered mn oxide by Potassium Fluoride an improvement for nanolayered mn oxide toward water oxidation
    International Journal of Hydrogen Energy, 2016
    Co-Authors: Mohammad Mahdi Najafpour, Seyedeh Maedeh Hosseini, Mohadeseh Zarei Ghobadi, Parvin Rafighi, Robabeh Bagheri, Zhenlun Song
    Abstract:

    Water splitting can store sustainable energies in the form of fuel (H2) and oxidant (O2). However, the efficiency of H2 production from the reaction is limited by the slow kinetics of the water oxidation. Herein the promising role of Fluoride on water-oxidizing activity of nanolayered Mn oxide is reported. The effects were studied for water oxidation in the presence of cerium(IV) ammonium nitrate. These experiments showed that the treatment of nanolayered Mn oxide by Potassium Fluoride increases water-oxidizing activity of these oxides in the presence of cerium(IV) ammonium nitrate approximately two times.