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Yoshiji Horikoshi - One of the best experts on this subject based on the ideXlab platform.

  • Successful growth of Cu2Se-free CuGaSe2 by Migration-Enhanced Epitaxy
    Journal of Vacuum Science & Technology. B. Nanotechnology and Microelectronics: Materials Processing Measurement and Phenomena, 2012
    Co-Authors: Miki Fujita, Tomohiro Sato, Tsuyoshi Kitada, Atsushi Kawaharazuka, Yoshiji Horikoshi
    Abstract:

    CuGaSe2 films were grown on GaAs (001) substrates by migration enhanced Epitaxy, where Cu + Ga and Se are alternately deposited. The in situ reflection high energy electron diffraction observation during growth revealed that the segregation of Cu2Se on CuGaSe2 can be detected by anomalous diffraction patterns. When the Cu2Se segregation takes place, a distorted pattern appears in both Cu + Ga and Se deposition periods. By optimizing the flux ratios, the anomalous diffraction disappears, and we succeeded in growing high quality CuGaSe2 single crystal layers free from Cu2Se segregation on GaAs (001) substrates. The authors also found that, in the CuGaSe2/GaAs wafers with Cu2Se segregation, a high density of voids is often observed at the substrate surface. These voids disappeared when the Cu2Se-free growth conditions were employed. Ga atoms near the GaAs substrate surface were probably drawn out by excess Cu atoms in the growing layer to form CuGaSe2, leading to the creation of voids with fairly large size.

  • Growth of CuGaSe2 Layers on Closely Lattice-Matched GaAs Substrates by Migration-Enhanced Epitaxy
    Japanese Journal of Applied Physics, 2011
    Co-Authors: Miki Fujita, Atsushi Kawaharazuka, Jiro Nishinaga, Klaus Ploog, Yoshiji Horikoshi
    Abstract:

    CuGaSe2 single-crystal films are grown on the As-stabilized (2×4) surface of (001) GaAs by Migration-Enhanced Epitaxy (MEE), where Cu+Ga and Se are alternately deposited. The growth process is monitored by refraction high-energy electron diffraction (RHEED) in the [110] azimuth. Under the Cu-enriched growth condition, a deformed 4-fold pattern is observed in both Cu+Ga and Se deposition periods. The deformed 4-fold pattern is found to be related to the segregation of Cu2Se on the CuGaSe2 surface as confirmed by the results of X-ray diffraction (XRD) measurement. By reducing the beam equivalent pressure of Cu (Cu-BEP), clear 4-fold patterns appear in both Cu+Ga and Se deposition periods instead of deformed 4-fold patterns. Further reduction of Cu-BEP results in clear 4- and 2-fold patterns for Cu+Ga and Se deposition periods. Under these growth conditions, Cu2Se-segregation-free CGS growth is achieved. Thus, the CuGaSe2 single-crystal layers without Cu2Se-segregation are successfully grown on GaAs(001) substrates by optimizing the Cu-BEP.

  • Area-selective Epitaxy of GaAs by Migration-Enhanced Epitaxy with As2 and As4 arsenic sources
    Applied Surface Science, 2008
    Co-Authors: Atsushi Kawaharazuka, Ippei Yoshiba, Yoshiji Horikoshi
    Abstract:

    Abstract We demonstrate area-selective Epitaxy by Migration-Enhanced Epitaxy with As2 and As4 as arsenic sources. The distinct whisker structure growing in [1 1 1]B direction is obtained when employing As2 as an arsenic source, while (1 1 1)B facet is formed with As4. The difference in the facet formation can be explained by the formation of As-trimer, which significantly reduces the growth rate of the (1 1 1)B surface. With As2, area-selective Epitaxy can be achieved at lower arsenic pressure condition, where less As-trimers are formed. Therefore, growth in the [1 1 1]B direction is enhanced.

  • Application of migration‐enhanced Epitaxy to novel semiconductor structures
    AIP Conference Proceedings, 2008
    Co-Authors: Yoshiji Horikoshi, Hiroshi Yamaguchi, S. Ramesh, Naoki Kobayashi
    Abstract:

    Abstract : Enhanced surface migration is essential to the growth of high quality epitaxial layers. In the growth of III-V compound semiconductors, surface migration is effectively enhanced by supplying group Ill atoms to the growing surface in the absence of group V atoms or molecules. In this situation, the lifetime of isolated group Ill atoms, which are quite mobile on the growing surface, is greatly increased resulting in these atoms migrating a large distance during growth. Migration-Enhanced Epitaxy (MEE) is based on this characteristic. MEE has proved useful for growing flat heterojunctions and for lowering the epitaxial growth temperature of III-V compound semiconductors. This paper describes the principle of MEE and its application to the growth of novel semiconductor structures such as GaAs/AlAs horizontal superlattices, ZnSe/GaAs superlattices, and (GaAs)l-x(Si2)x,/GaAs superlattices.

  • Characterization of heavily Sn-doped GaAs grown by Migration-Enhanced Epitaxy
    Journal of Crystal Growth, 2007
    Co-Authors: Tosaporn Chavanapranee, Yoshiji Horikoshi
    Abstract:

    Abstract The saturation of electron concentration and mobility at high doping concentration observed in the samples grown by low-temperature Migration-Enhanced Epitaxy (MEE) is found to be strongly related to the morphology change in the film. The structural characteristics of the heavily Sn-doped GaAs have been further investigated by means of X-ray diffraction (XRD) measurement and transmission electron microscopy (TEM). The results indicate that the (GaAs) 1– x (Sn 2 ) x alloy is formed in the Sn-doped GaAs with the doping concentration higher than 1×10 19  cm −3 . However, when the Sn concentration exceeds 1×10 21  cm −3 , the formation of Sn-rich clusters becomes dominant. This formation of (GaAs) 1– x (Sn 2 ) x alloy and Sn clusters is found to be responsible for the saturation of the electron concentration and mobility in the heavily doped samples.

Won Jun Choi - One of the best experts on this subject based on the ideXlab platform.

Shun-ichi Gonda - One of the best experts on this subject based on the ideXlab platform.

  • Gas source molecular beam Epitaxy/migration enhanced Epitaxy growth of InAs/AlSb superlattices
    Journal of Applied Physics, 1993
    Co-Authors: Masumichi Seta, Hajime Asahi, Kumiko Asami, Shun-ichi Gonda
    Abstract:

    We report on the gas source molecular beam Epitaxy/migration enhanced Epitaxy (MEE) growth of InAs/AlSb superlattices. The incorporation behavior of constituent group III and group V atoms during growth is investigated in detail using reflection high energy electron diffraction. In and Sb atoms are found to move towards the surface during MEE growth, although the movement of In atoms can be reduced by lowering the growth temperature. Raman scattering measurement of InAs/AlSb superlattices shows that the formation of atomically controlled heterointerfaces (InSb‐ or AlAs‐type interfaces in InAs/AlSb superlattices) is difficult. However, photoluminescence (PL) measurement shows that the optical properties of quantum well structures are strongly dependent on the shutter sequence at the interfaces. 77 K PL from InAs/AlSb quantum well structures with an InSb‐type interface shutter sequence is one order of magnitude stronger than that of the AlAs‐type interface.

  • Atomically controlled InGaAs/InP superlattices grown by gas source MEE (migration enhanced Epitaxy)
    Journal of Crystal Growth, 1993
    Co-Authors: Hajime Asahi, Kumiko Asami, Teruaki Kohara, R.k. Soni, Shuichi Emura, Shun-ichi Gonda
    Abstract:

    Abstract Atomically controlled InGaAs/InP SL structures having different types of heterointerfaces are grown on (001)InP substrates at 350°C gas source MEE (migration enhanced Epitaxy). RHEED intensity traces exhibit the same shape at the positions of the same type of heterointerfaces, indicating the formation of the desired heterointerfaces. The Raman spectrum from the SL, having only the InAs-type heterointerfaces, is characterized by the absence of GaP-like LO phonon clearly suggesting the formation of only the InAs-type heterointerfaces, while the SL having InGaP-type interfaces indeed shows the presence of GaP-like LO phonon peak. 4.2 K photoluminescence (PL) spectra for the InGaAs/InP quantum well (QW) structures show a very narrow line width comparable to the narrowest line width reported so far. Furthermore, the PL peak energy variation with well thickness clearly depends on the heterointerface type.

  • Influence of hydrogen on the step flow growth of GaAs on vicinal surfaces by gas‐source migration enhanced Epitaxy
    Applied Physics Letters, 1992
    Co-Authors: Hajime Asahi, Soon Jae Yu, Tadaaki Kaneko, T. Hisaka, Yasutoshi Okuno, Shun-ichi Gonda
    Abstract:

    Step flow growth of GaAs on the vicinal surfaces by gas‐source migration enhanced Epitaxy (MEE), the combination of gas‐source molecular beam Epitaxy and MEE, is studied with the reflection high‐energy electron diffraction (RHEED) intensity oscillation. It is found that the use of the thermally cracked AsH3 instead of solid As (As4) as an As source enhances step flow growth of GaAs on the (001) surface misoriented toward the [110] direction. The same tendency is also observed in the MEE growth using As4 under the hydrogen supply. It is considered that the enhancement of step flow growth in the gas‐source MEE is caused by the hydrogen atoms terminated at the steps.

  • Gas source MEE (migration enhanced Epitaxy) growth of InP
    Journal of Crystal Growth, 1991
    Co-Authors: Nobuyuki Takeyasu, Hajime Asahi, Soon Jae Yu, Kumiko Asami, Tadaaki Kaneko, Shun-ichi Gonda
    Abstract:

    Abstract High-quality InP layers are grown by gas source MEE (migration enhanced Epitaxy) method at 350°C. It is found that even at a substrate temperature as low as 350°C, the desorption of some amount of phosphorus from the InP surface occurs when the PH 3 flow is interrupted, although the RHEED pattern is still showing the (2×4) reconstructions. As a result, the perfectly alternating supply of indium and phosphorus can be achieved only when PH 3 is supplied with a proper interruption time before the supply of In. It is also found that InP layers grown by gas source MEE at 350°C have optical properties equal to or better than those grown by conventional gas source MBE (molecular beam Epitaxy) at 470°C.

J. Singh - One of the best experts on this subject based on the ideXlab platform.

D. L. Miller - One of the best experts on this subject based on the ideXlab platform.

  • Electrical properties of low-temperature GaAs grown by molecular beam Epitaxy and migration enhanced Epitaxy
    Journal of Electronic Materials, 1993
    Co-Authors: Kai Zhang, D. L. Miller
    Abstract:

    Measurements on low-temperature GaAs epitaxial layers (LT-GaAs) grown by molecular beam Epitaxy and migration enhanced Epitaxy showed that the excess arsenic incorporated during growth played a crucial role in determining their electrical properties. The electrical transport in LT-GaAs grown by a standard molecular beam Epitaxy proceeded mainly via a hopping process, which showed a higher activation energy and onset temperature than those usually observed in lightly doped semiconductors. Using migration enhanced Epitaxy to grow LT-GaAs, we were able to substantially reduce the density of As-rich defects and to achieve a good Hall mobility in Be-doped LT-GaAs. The study presented here indicates that, with controlled excess arsenic incorporation during growth, LT-GaAs can vary in a range of conduction properties and thus can be engineered for different device applications.

  • Low‐temperature migration enhanced Epitaxy of base material for AlGaAs/GaAs heterojunction bipolar transistors
    Applied Physics Letters, 1993
    Co-Authors: Kai Zhang, D. L. Miller, Jianming Fu, Der-woei Wu, Mike Fukuda, Stephen Schauer
    Abstract:

    Migration enhanced Epitaxy (MEE) was used in this work to grow p+‐GaAs at the substrate temperature of 300 °C for the base of AlGaAs/GaAs heterojunction bipolar transistors. The results indicated that the low‐temperature MEE‐grown p+‐GaAs epitaxial layers (p=1×1019–1×1020 cm−3) exhibited a crystalline quality comparable to those grown by standard MBE at a substrate temperature of 570 °C. AlGaAs/GaAs HBTs with low‐temperature MEE‐grown bases doped at p≊2×1019 cm−3 were fabricated by using a self‐alignment technique. For the devices with the conventional MBE‐grown base, secondary ion mass spectroscopy depth profiles showed a significant Be diffusion into the AlGaAs emitter and as a consequence, the devices showed no current gain. For the devices with the low‐temperature MBE‐grown base, there was a negligible Be penetration into the emitter and the devices exhibited a common‐emitter dc current gain of 13.

  • Scanning tunneling microscope study of GaAs(001) surfaces grown by migration enhanced Epitaxy
    Journal of Vacuum Science & Technology B, 1993
    Co-Authors: M. C. Gallagher, Jianming Fu, Roy F. Willis, D. L. Miller
    Abstract:

    We report an investigation of the morphology of p‐type GaAs(001) surfaces using scanning tunneling microscopy (STM). The substrates were prepared using two methods: migration enhanced Epitaxy (MEE) and standard molecular‐beam Epitaxy (MBE). The STM measurements were performed ex situ using As decapping. Analysis indicates that the overall step density of the MEE samples decreases as the growth temperature is increased. Nominally flat samples grown at 300 °C exhibited step densities of 10.5 steps/1000 A along [110] dropping to 2.5 steps at 580 °C. MEE samples exhibited a lower step density than MBE samples. However as‐grown surfaces exhibited a larger distribution of step heights. Annealing the samples reduced the step height distribution exposing fewer atomic layers. Samples grown by MEE at 580 °C and annealed for 2 min displayed the lowest step density and the narrowest step height distribution. All samples displayed an anisotropic step density. We found a ratio of A‐type to B‐type steps of between 2 and...

  • Migration‐enhanced Epitaxy of doped GaAs on (111)B and (100)GaAs substrates
    Journal of Vacuum Science & Technology B, 1992
    Co-Authors: Jianming Fu, Kai Zhang, D. L. Miller
    Abstract:

    Si‐doped n‐type GaAs and Be‐doped p‐type GaAs have been grown on (111)B oriented GaAs substrates using the migration‐enhanced Epitaxy (MEE) technique, in which arsenic and gallium are deposited separately. The mobilities and carrier densities have been compared with GaAs grown by MEE and conventional Epitaxy on GaAs (100) substrates. Under migration enhanced conditions, the range of substrate temperatures and arsenic fluxes to obtain smooth surfaces and good mobilities is wider than for conventional molecular‐beam Epitaxy, for both substrate orientations. High‐quality doped GaAs material was obtained at substrate temperature as low as 400–450 °C on (111)B substrates.

  • Be doped GaAs grown by migration enhanced Epitaxy at low substrate temperature
    Journal of Electronic Materials, 1992
    Co-Authors: Kai Zhang, S. S. Bose, D. L. Miller
    Abstract:

    Conductive Be doped GaAs grown by molecular beam Epitaxy at low substrate temperatures (300° C) was obtained for the first time by using migration enhanced Epitaxy (MEE) without subsequent annealing. The layers were characterized using Hall effect, double crystal x-ray diffraction, and photoluminescence. With low arsenic exposure, the low temperature MEE layers doped with Be had the same carrier density and similar luminescent efficiency as layers grown by conventional MBE at 580° C. Mobility at 77 K was reduced somewhat for layers doped at 2 × 10^17cm^−3, which also exhibited hopping conductivity below 40 K. Double crystal x-ray diffraction showed that low temperature MEE samples grown at low As exposure had the narrow linewidth associated with conventional MBE material grown at 580° C, unlike layers grown by conventional MBE at low temperatures, which exhibit an expansion in lattice parameter.